Strength of correlation effects in the electronic structure of iron

The strength of electronic correlation effects in the spin-dependent electronic structure of ferromagnetic bcc Fe(110) has been investigated by means of spin and angle-resolved photoemission spectroscopy. The experimental results are compared to theoretical calculations within the three-body scatter...

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Veröffentlicht in:Physical review letters 2009-12, Vol.103 (26), p.267203-267203, Article 267203
Hauptverfasser: Sánchez-Barriga, J, Fink, J, Boni, V, Di Marco, I, Braun, J, Minár, J, Varykhalov, A, Rader, O, Bellini, V, Manghi, F, Ebert, H, Katsnelson, M I, Lichtenstein, A I, Eriksson, O, Eberhardt, W, Dürr, H A
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Sprache:eng
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Zusammenfassung:The strength of electronic correlation effects in the spin-dependent electronic structure of ferromagnetic bcc Fe(110) has been investigated by means of spin and angle-resolved photoemission spectroscopy. The experimental results are compared to theoretical calculations within the three-body scattering approximation and within the dynamical mean-field theory, together with one-step model calculations of the photoemission process. This comparison indicates that the present state of the art many-body calculations, although improving the description of correlation effects in Fe, give too small mass renormalizations and scattering rates thus demanding more refined many-body theories including nonlocal fluctuations.
ISSN:0031-9007
1079-7114
1079-7114
DOI:10.1103/physrevlett.103.267203