Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption

Periodic metal-dielectric structures attract substantial interest since it was previously proposed that the spontaneous emission amplification rates (the Purcell factor) in such structures can reach enormous values up to 10 5 . However, the role of absorption in real metals has not been thoroughly c...

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Veröffentlicht in:Scientific reports 2019-07, Vol.9 (1), p.9604-9, Article 9604
Hauptverfasser: Morozov, Konstantin M., Ivanov, Konstantin A., de Sa Pereira, Daniel, Menelaou, Christopher, Monkman, Andrew P., Pozina, Galia, Kaliteevski, Mikhail A.
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Sprache:eng
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Zusammenfassung:Periodic metal-dielectric structures attract substantial interest since it was previously proposed that the spontaneous emission amplification rates (the Purcell factor) in such structures can reach enormous values up to 10 5 . However, the role of absorption in real metals has not been thoroughly considered. We provide a theoretical analysis showing that absorption leads to diminishing values of Purcell factor. We also suggest that using emitting organic compounds such as CBP (4,4-Bis(N-carbazolyl)-1,1-biphenyl) can lead to a moderate increase of about an order of magnitude in the Purcell factor. Defining the experimentally measured Purcell factor as a ratio between the excited state lifetimes in bare CBP and in periodic structure, this increase in the fabricated periodic structure is demonstrated through a 4–8 times decrease in excited state radiative lifetime compared to a bare organic material in a wide emission spectrum.
ISSN:2045-2322
2045-2322
DOI:10.1038/s41598-019-46071-5