Infrared Spectroscopy of CH4/N2 and C2Hm/N2 (m=2,4,6) Gas Mixtures in a Dielectric Barrier Discharge

Infrared Spectroscopy of CH4/N2 and C2Hm/N2 (m=2,4,6) Gas Mixtures in a Dielectric Barrier Discharge

Fourier transform infrared spectroscopy of CH 4 / N 2 and C 2 H m / N 2 ( m = 2 , 4 , 6 ) gas mixtures in a medium pressure (300 mbar) dielectric barrier discharge was performed. Consumption of the initial gas and formation of other hydrocarbon and of nitrogen-containing HCN and NH 3 molecules was o...

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Veröffentlicht in:Plasma chemistry and plasma processing 2014, Vol.34 (5), p.1157-1170
Hauptverfasser: Thejaswini, H. C., Peglow, Sandra, Sushkov, Vladimir, Hippler, Rainer
Format: Artikel
Sprache:eng
Schlagworte:
Characterization and Evaluation of Materials
Chemistry
Chemistry and Materials Science
Classical Mechanics
Inorganic Chemistry
Mechanical Engineering
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Zusammenfassung:Fourier transform infrared spectroscopy of CH 4 / N 2 and C 2 H m / N 2 ( m = 2 , 4 , 6 ) gas mixtures in a medium pressure (300 mbar) dielectric barrier discharge was performed. Consumption of the initial gas and formation of other hydrocarbon and of nitrogen-containing HCN and NH 3 molecules was observed. NH 3 formation was further confirmed by laser absorption measurements. The experimental result for NH 3 is at variance with simulation results.
ISSN:0272-4324
1572-8986
DOI:10.1007/s11090-014-9557-x