Electrical gating of superconducting NbSe2 using SrTiO3-based field-effect transistors

We report on electrical gating of superconducting bilayer NbSe2 using dual-gate field-effect transistors constructed by the van der Waals assembly of mechanically exfoliated NbSe2 and SrTiO3 thin films grown by molecular beam epitaxy. Charge carrier doping, but not a pure electric field, was found to induce changes to the superconducting resistive transition, reaching a 190 mK modulation of the critical temperature and excluding the Rashba effect. The phase space for the superconducting state beyond the Pauli limit under in-plane magnetic fields expands when the critical temperature is enhanced. Quantitative comparison with theory suggests the presence of intervalley scattering, which competes with Ising spin–orbit coupling to set the superconducting-normal phase boundary. The gating method demonstrated here may be applied to study other van der Waals layered superconductors.