Excellent energy storage properties, domain mechanism, and temperature stability of lead-free BaTiO3-Bi(Mg1/2Sn1/2)O3 bulk ferroelectrics
Pulsed power systems require high-performance capacitors with high energy storage density. In this work, (1 − x)BaTiO3-xBi(Mg1/2Sn1/2)O3 ferroelectric ceramics were synthesized in a solid-state solution. The sample of x = 0.12 (0.88BT-0.12BMS) has excellent energy storage density, wide temperature,...
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| Veröffentlicht in: | Applied physics letters 2023-04, Vol.122 (17) |
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| creator | Qie, Dan Tang, Zhenhua Fang, Junlin Yao, Dijie Zhang, Li Jiang, Yan-Ping Sun, Qi-Jun Zhang, Dan Fan, Jing-Min Tang, Xin-Gui Liu, Qiu-Xiang Zhou, Yi-Chun |
| description | Pulsed power systems require high-performance capacitors with high energy storage density. In this work, (1 − x)BaTiO3-xBi(Mg1/2Sn1/2)O3 ferroelectric ceramics were synthesized in a solid-state solution. The sample of x = 0.12 (0.88BT-0.12BMS) has excellent energy storage density, wide temperature, and wide frequency stability. The excellent energy density of 4.87 J/cm3 at 315 kV/cm and the energy efficiency of 72% at room temperature for 0.88BT-0.12BMS ceramics were achieved. Furthermore, the 0.88BT-0.12BMS ceramics demonstrated well temperature stabilities in the range of 20–100 °C and very good frequency stability in the range of 1–100 Hz. Through pulsed charging–discharging testing, the current density is calculated as 314.01 A/cm2, and the power density is 21.98 MW/cm3. Moreover, the oxygen vacancies' defects and ferroelectric domain mechanism for enhanced breakdown strength as well as high energy density were discussed. These findings broaden the horizon for lead-free dielectrics and show promising applications for pulse power capacitors. |
| doi_str_mv | 10.1063/5.0137616 |
| format | Article |
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In this work, (1 − x)BaTiO3-xBi(Mg1/2Sn1/2)O3 ferroelectric ceramics were synthesized in a solid-state solution. The sample of x = 0.12 (0.88BT-0.12BMS) has excellent energy storage density, wide temperature, and wide frequency stability. The excellent energy density of 4.87 J/cm3 at 315 kV/cm and the energy efficiency of 72% at room temperature for 0.88BT-0.12BMS ceramics were achieved. Furthermore, the 0.88BT-0.12BMS ceramics demonstrated well temperature stabilities in the range of 20–100 °C and very good frequency stability in the range of 1–100 Hz. Through pulsed charging–discharging testing, the current density is calculated as 314.01 A/cm2, and the power density is 21.98 MW/cm3. Moreover, the oxygen vacancies' defects and ferroelectric domain mechanism for enhanced breakdown strength as well as high energy density were discussed. These findings broaden the horizon for lead-free dielectrics and show promising applications for pulse power capacitors.</description><identifier>ISSN: 0003-6951</identifier><identifier>EISSN: 1077-3118</identifier><identifier>DOI: 10.1063/5.0137616</identifier><identifier>CODEN: APPLAB</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>Applied physics ; Barium titanates ; Capacitors ; Ceramics ; Energy storage ; Ferroelectric domains ; Ferroelectric materials ; Ferroelectricity ; Frequency stability ; Lead free ; Room temperature</subject><ispartof>Applied physics letters, 2023-04, Vol.122 (17)</ispartof><rights>Author(s)</rights><rights>2023 Author(s). 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In this work, (1 − x)BaTiO3-xBi(Mg1/2Sn1/2)O3 ferroelectric ceramics were synthesized in a solid-state solution. The sample of x = 0.12 (0.88BT-0.12BMS) has excellent energy storage density, wide temperature, and wide frequency stability. The excellent energy density of 4.87 J/cm3 at 315 kV/cm and the energy efficiency of 72% at room temperature for 0.88BT-0.12BMS ceramics were achieved. Furthermore, the 0.88BT-0.12BMS ceramics demonstrated well temperature stabilities in the range of 20–100 °C and very good frequency stability in the range of 1–100 Hz. Through pulsed charging–discharging testing, the current density is calculated as 314.01 A/cm2, and the power density is 21.98 MW/cm3. Moreover, the oxygen vacancies' defects and ferroelectric domain mechanism for enhanced breakdown strength as well as high energy density were discussed. These findings broaden the horizon for lead-free dielectrics and show promising applications for pulse power capacitors.</description><subject>Applied physics</subject><subject>Barium titanates</subject><subject>Capacitors</subject><subject>Ceramics</subject><subject>Energy storage</subject><subject>Ferroelectric domains</subject><subject>Ferroelectric materials</subject><subject>Ferroelectricity</subject><subject>Frequency stability</subject><subject>Lead free</subject><subject>Room temperature</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNp9kM9KAzEQxoMoWKsH3yDgRaWrycYk7dFK_QNKD-p5yWYnNbqb1CQr9hF8ayMVPQheZpjhN9_wfQjtU3JCiWCn_IRQJgUVG2hAiZQFo3S8iQaEEFaICafbaCfG5zzykrEB-pi9a2hbcAmDg7BY4Zh8UAvAy-CXEJKFOMKN75R1uAP9pJyN3Qgr1-AEXSZU6gPkK1Xb1qYV9ga3oJrCBAA8VQ92zoqpPbxb0NPy3uVyNGe47tsXbCAEDy3oFKyOu2jLqDbC3ncfosfL2cPFdXE7v7q5OL8tNBNlKqBRxmhSS8FLTiXnRjA-yS4bxqioz0hTSsnHQue1UTChLMdAGimJqbNnwoboYK2bDb72EFP17Pvg8suqHBNRsjNGy0wdrSkdfIwBTLUMtlNhVVFSfSVd8eo76cwer9mobVLJevcDv_nwC1bLxvwH_1X-BNVAixQ</recordid><startdate>20230424</startdate><enddate>20230424</enddate><creator>Qie, Dan</creator><creator>Tang, Zhenhua</creator><creator>Fang, Junlin</creator><creator>Yao, Dijie</creator><creator>Zhang, Li</creator><creator>Jiang, Yan-Ping</creator><creator>Sun, Qi-Jun</creator><creator>Zhang, Dan</creator><creator>Fan, Jing-Min</creator><creator>Tang, Xin-Gui</creator><creator>Liu, Qiu-Xiang</creator><creator>Zhou, Yi-Chun</creator><general>American Institute of Physics</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0002-1500-8668</orcidid><orcidid>https://orcid.org/0000-0003-4557-1707</orcidid><orcidid>https://orcid.org/0000-0003-1321-5687</orcidid><orcidid>https://orcid.org/0000-0001-9821-6042</orcidid><orcidid>https://orcid.org/0000-0001-6028-5544</orcidid><orcidid>https://orcid.org/0000-0002-0679-8549</orcidid><orcidid>https://orcid.org/0000-0001-6429-2098</orcidid><orcidid>https://orcid.org/0000-0003-1013-0004</orcidid><orcidid>https://orcid.org/0000-0002-5789-9059</orcidid><orcidid>https://orcid.org/0000-0002-4440-3413</orcidid></search><sort><creationdate>20230424</creationdate><title>Excellent energy storage properties, domain mechanism, and temperature stability of lead-free BaTiO3-Bi(Mg1/2Sn1/2)O3 bulk ferroelectrics</title><author>Qie, Dan ; Tang, Zhenhua ; Fang, Junlin ; Yao, Dijie ; Zhang, Li ; Jiang, Yan-Ping ; Sun, Qi-Jun ; Zhang, Dan ; Fan, Jing-Min ; Tang, Xin-Gui ; Liu, Qiu-Xiang ; Zhou, Yi-Chun</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c362t-edaffc0b765251755f6359311d3316b40d277586c635fae9131070d770fb05203</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Applied physics</topic><topic>Barium titanates</topic><topic>Capacitors</topic><topic>Ceramics</topic><topic>Energy storage</topic><topic>Ferroelectric domains</topic><topic>Ferroelectric materials</topic><topic>Ferroelectricity</topic><topic>Frequency stability</topic><topic>Lead free</topic><topic>Room temperature</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Qie, Dan</creatorcontrib><creatorcontrib>Tang, Zhenhua</creatorcontrib><creatorcontrib>Fang, Junlin</creatorcontrib><creatorcontrib>Yao, Dijie</creatorcontrib><creatorcontrib>Zhang, Li</creatorcontrib><creatorcontrib>Jiang, Yan-Ping</creatorcontrib><creatorcontrib>Sun, Qi-Jun</creatorcontrib><creatorcontrib>Zhang, Dan</creatorcontrib><creatorcontrib>Fan, Jing-Min</creatorcontrib><creatorcontrib>Tang, Xin-Gui</creatorcontrib><creatorcontrib>Liu, Qiu-Xiang</creatorcontrib><creatorcontrib>Zhou, Yi-Chun</creatorcontrib><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Qie, Dan</au><au>Tang, Zhenhua</au><au>Fang, Junlin</au><au>Yao, Dijie</au><au>Zhang, Li</au><au>Jiang, Yan-Ping</au><au>Sun, Qi-Jun</au><au>Zhang, Dan</au><au>Fan, Jing-Min</au><au>Tang, Xin-Gui</au><au>Liu, Qiu-Xiang</au><au>Zhou, Yi-Chun</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Excellent energy storage properties, domain mechanism, and temperature stability of lead-free BaTiO3-Bi(Mg1/2Sn1/2)O3 bulk ferroelectrics</atitle><jtitle>Applied physics letters</jtitle><date>2023-04-24</date><risdate>2023</risdate><volume>122</volume><issue>17</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><coden>APPLAB</coden><abstract>Pulsed power systems require high-performance capacitors with high energy storage density. In this work, (1 − x)BaTiO3-xBi(Mg1/2Sn1/2)O3 ferroelectric ceramics were synthesized in a solid-state solution. The sample of x = 0.12 (0.88BT-0.12BMS) has excellent energy storage density, wide temperature, and wide frequency stability. The excellent energy density of 4.87 J/cm3 at 315 kV/cm and the energy efficiency of 72% at room temperature for 0.88BT-0.12BMS ceramics were achieved. Furthermore, the 0.88BT-0.12BMS ceramics demonstrated well temperature stabilities in the range of 20–100 °C and very good frequency stability in the range of 1–100 Hz. Through pulsed charging–discharging testing, the current density is calculated as 314.01 A/cm2, and the power density is 21.98 MW/cm3. Moreover, the oxygen vacancies' defects and ferroelectric domain mechanism for enhanced breakdown strength as well as high energy density were discussed. 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| source | AIP Journals Complete; Alma/SFX Local Collection |
| subjects | Applied physics Barium titanates Capacitors Ceramics Energy storage Ferroelectric domains Ferroelectric materials Ferroelectricity Frequency stability Lead free Room temperature |
| title | Excellent energy storage properties, domain mechanism, and temperature stability of lead-free BaTiO3-Bi(Mg1/2Sn1/2)O3 bulk ferroelectrics |
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