Single-atom alloy Ir/Ni catalyst boosts CO methanation mechanochemistry

A new catalytic approach is pioneered to achieve CO 2 methanation via a single atom alloy Ir/Ni catalyst using a ball-milling method. This Ir/Ni catalyst exhibits a TOF CH4 of 10244 h −1 and a 220 h lifetime at 350 °C without deactivation, illustrating excellent catalytic efficiency in the presence...

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Veröffentlicht in:Nanoscale horizons 2023-06, Vol.8 (7), p.852-858
Hauptverfasser: Tu, Rui, Zhang, Yujie, Xu, Yuchun, Yang, Junxia, Zhang, Ling, Lv, Keran, Ren, Guoqing, Zhai, Shengliang, Yu, Tie, Deng, Weiqiao
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Zusammenfassung:A new catalytic approach is pioneered to achieve CO 2 methanation via a single atom alloy Ir/Ni catalyst using a ball-milling method. This Ir/Ni catalyst exhibits a TOF CH4 of 10244 h −1 and a 220 h lifetime at 350 °C without deactivation, illustrating excellent catalytic efficiency in the presence of mechanical energy. A new catalytic approach is pioneered to achieve CO 2 methanation via a single atom alloy Ir/Ni catalyst using a ball-milling method.
ISSN:2055-6756
2055-6764
DOI:10.1039/d3nh00040k