Ultrabright carbon dots as a fluorescent nano sensor for Pb detection

In this work, we synthesized ultrabright carbon dots (U-CDs) with photoluminescence quantum yield (PLQY) up to ∼100% using CA and EDA as precursors. When studying their interaction with the Pb 2+ ion, we found that the PL quenching degree is independent of the U-CDs concentration. This feature provi...

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Veröffentlicht in:RSC advances 2022-08, Vol.12 (37), p.2439-24396
Hauptverfasser: Long, Xiang, Li, Ruixue, Xiang, Jiamei, Wu, Shaogui, Wang, Jiayang
Format: Artikel
Sprache:eng
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Zusammenfassung:In this work, we synthesized ultrabright carbon dots (U-CDs) with photoluminescence quantum yield (PLQY) up to ∼100% using CA and EDA as precursors. When studying their interaction with the Pb 2+ ion, we found that the PL quenching degree is independent of the U-CDs concentration. This feature provides great convenience for practical detection, which allows the standard curve determination and practical detection to be conducted under different U-CDs concentrations with detection error less than 20%. Based on the experimental observations, a possible mechanism is proposed to explain this phenomenon. To our best knowledge, this work has never been reported before and provides a new idea for the design of novel fluorescent sensors. An interesting phenomenon of ultrabright fluorescent carbon dots as a metal ion sensor for Pb 2+ ion detection.
ISSN:2046-2069
DOI:10.1039/d2ra03591j