Scheme MoS/TiO/graphene nanohybrid photocatalysts for visible light-induced degradation for highly efficient water disinfection and antibacterial activity
We fabricated MoS 2 /TiO 2 /graphene (MTG) nanohybrids using a hydrothermal process in the preparation of heterostructure photocatalysts. The MTG nanohybrids exhibited high stability, large specific surface area, and visible light response. The heterostructure nanohybrids were effective in the visib...
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Veröffentlicht in: | New journal of chemistry 2022-07, Vol.46 (29), p.14159-14169 |
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Zusammenfassung: | We fabricated MoS
2
/TiO
2
/graphene (MTG) nanohybrids using a hydrothermal process in the preparation of heterostructure photocatalysts. The MTG nanohybrids exhibited high stability, large specific surface area, and visible light response. The heterostructure nanohybrids were effective in the visible-light photodegradation of tetracycline (TC), rhodamine B (RhB), and congo red (CR), as well as Pb(
ii
) reduction. The nanohybrids exhibited a photocatalytic TC removal capability of 94.5% with 60 min of visible light irradiation. Suppressing the recombination of photoexcited electron-hole pairs enhanced the removal of environmental pollutants. The MTG nanohybrids also displayed photocatalytic reduction of Pb(
ii
), approximately 10-15 times that of bare MoS
2
and TiO
2
samples. The nanohybrids also showed efficient photocatalytic antibacterial performance, killing 99.9% of
E. coli
in 10 min, thus demonstrating environmental friendliness in water disinfection. The results clearly demonstrated promising nanohybrids for the photocatalytic removal of a wide variety of contaminants, such as hazardous organic chemicals, heavy metals, and pathogenic microbes, under visible light irradiation.
A new
Z
-scheme MoS
2
/TiO
2
/graphene nanohybrid effectively degraded antibiotics, heavy metals and microorganisms under visible irradiation. |
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ISSN: | 1144-0546 1369-9261 |
DOI: | 10.1039/d2nj01824a |