Acetic acid formation from methane and carbon dioxide non-thermal plasma reactions towards an effective carbon fixation

While direct CH 3 COOH formation from CH 4 and CO 2 in a non-equilibrium condition is an ideal process, a dielectric-barrier discharge plasma reaction in the presence of CO 2 and isotopic CH 4 ( 13 CH 4 ) revealed that the primly produced CH 3 COOH can comprise both CH 4 -derived carbons ( i.e. , no...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:New journal of chemistry 2022-05, Vol.46 (17), p.7855-7858
Hauptverfasser: Nishimura, Naoyuki, Akaogi, Takayuki, Onishi, Kazuhiro, Tojo, Masahiro
Format: Artikel
Sprache:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Beschreibung
Zusammenfassung:While direct CH 3 COOH formation from CH 4 and CO 2 in a non-equilibrium condition is an ideal process, a dielectric-barrier discharge plasma reaction in the presence of CO 2 and isotopic CH 4 ( 13 CH 4 ) revealed that the primly produced CH 3 COOH can comprise both CH 4 -derived carbons ( i.e. , no CO 2 -derived carbon), indicating the importance of a particular CO 2 activation control in non-thermal plasma for an effective carbon fixation. A non-thermal plasma reaction with CO 2 and isotopic CH 4 revealed that the primly produced CH 3 COOH could comprise both CH 4 -derived carbons, indicating the importance of a particular CO 2 activation control for an effective carbon fixation.
ISSN:1144-0546
1369-9261
DOI:10.1039/d2nj00409g