Probing FeSi, a d -electron topological Kondo insulator candidate, with magnetic field, pressure, and microwaves
Recently, evidence for a conducting surface state (CSS) below 19 K was reported for the correlated -electron small gap semiconductor FeSi. In the work reported herein, the CSS and the bulk phase of FeSi were probed via electrical resistivity ρ measurements as a function of temperature , magnetic fie...
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creator | Breindel, Alexander J Deng, Yuhang Moir, Camilla M Fang, Yuankan Ran, Sheng Lou, Hongbo Li, Shubin Zeng, Qiaoshi Shu, Lei Wolowiec, Christian T Schuller, Ivan K Rosa, Priscila F S Fisk, Zachary Singleton, John Maple, M Brian |
description | Recently, evidence for a conducting surface state (CSS) below 19 K was reported for the correlated
-electron small gap semiconductor FeSi. In the work reported herein, the CSS and the bulk phase of FeSi were probed via electrical resistivity ρ measurements as a function of temperature
, magnetic field
to 60 T, and pressure
to 7.6 GPa, and by means of a magnetic field-modulated microwave spectroscopy (MFMMS) technique. The properties of FeSi were also compared with those of the Kondo insulator SmB
to address the question of whether FeSi is a
-electron analogue of an
-electron Kondo insulator and, in addition, a "topological Kondo insulator" (TKI). The overall behavior of the magnetoresistance of FeSi at temperatures above and below the onset temperature
= 19 K of the CSS is similar to that of SmB
. The two energy gaps, inferred from the ρ(
) data in the semiconducting regime, increase with pressure up to about 7 GPa, followed by a drop which coincides with a sharp suppression of
. Several studies of ρ(
) under pressure on SmB
reveal behavior similar to that of FeSi in which the two energy gaps vanish at a critical pressure near the pressure at which
vanishes, although the energy gaps in SmB
initially decrease with pressure, whereas in FeSi they increase with pressure. The MFMMS measurements showed a sharp feature at
≈ 19 K for FeSi, which could be due to ferromagnetic ordering of the CSS. However, no such feature was observed at
≈ 4.5 K for SmB
. |
doi_str_mv | 10.1073/pnas.2216367120 |
format | Article |
fullrecord | <record><control><sourceid>proquest_pubme</sourceid><recordid>TN_cdi_pubmedcentral_primary_oai_pubmedcentral_nih_gov_9974408</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2779948086</sourcerecordid><originalsourceid>FETCH-LOGICAL-c448t-98df5f2f7d993131b0925a027e7baaf7bacd0951caa64c1991d7c214ed7bd1973</originalsourceid><addsrcrecordid>eNpdkc9vFCEcxYmxsWv17M0Qe_Gw0wLDDsPFxDStNjbRRD2T7wCzS8PACEwb_3vZbK0_OMDh--HBew-hV5ScUSLa8zlAPmOMdm0nKCNP0IoSSZuOS_IUrQhhouk548foec63hBC56ckzdFxpSetaoflLioMLW3xlv7o1BmxwY73VJcWAS5yjj1unweNPMZiIXciLhxIT1hCMM1DsGt-7ssMTbIMtTuPRWW_WeE425yXVcQXx5HSK93Bn8wt0NILP9uXDeYK-X11-u_jY3Hz-cH3x_qbRnPelkb0ZNyMbhZGypS0diGQbqH6sGADGumlT3VAN0HFNpaRGaEa5NWIwVIr2BL076M7LMFmjbSgJvJqTmyD9VBGc-ncS3E5t452SUnBO-irw5iAQc3Eqa1es3ukYQg1HUcl438oKvX14JcUfi81FTS5r6z0EG5esmBCCUCbIHj39D72NSwo1gz0lJe9J31Xq_EDVvHJOdnz8MSVqX7naV67-VF5vvP7b6CP_u-P2F_BxqLA</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2779948086</pqid></control><display><type>article</type><title>Probing FeSi, a d -electron topological Kondo insulator candidate, with magnetic field, pressure, and microwaves</title><source>PubMed Central</source><source>Alma/SFX Local Collection</source><source>Free Full-Text Journals in Chemistry</source><creator>Breindel, Alexander J ; Deng, Yuhang ; Moir, Camilla M ; Fang, Yuankan ; Ran, Sheng ; Lou, Hongbo ; Li, Shubin ; Zeng, Qiaoshi ; Shu, Lei ; Wolowiec, Christian T ; Schuller, Ivan K ; Rosa, Priscila F S ; Fisk, Zachary ; Singleton, John ; Maple, M Brian</creator><creatorcontrib>Breindel, Alexander J ; Deng, Yuhang ; Moir, Camilla M ; Fang, Yuankan ; Ran, Sheng ; Lou, Hongbo ; Li, Shubin ; Zeng, Qiaoshi ; Shu, Lei ; Wolowiec, Christian T ; Schuller, Ivan K ; Rosa, Priscila F S ; Fisk, Zachary ; Singleton, John ; Maple, M Brian ; Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)</creatorcontrib><description>Recently, evidence for a conducting surface state (CSS) below 19 K was reported for the correlated
-electron small gap semiconductor FeSi. In the work reported herein, the CSS and the bulk phase of FeSi were probed via electrical resistivity ρ measurements as a function of temperature
, magnetic field
to 60 T, and pressure
to 7.6 GPa, and by means of a magnetic field-modulated microwave spectroscopy (MFMMS) technique. The properties of FeSi were also compared with those of the Kondo insulator SmB
to address the question of whether FeSi is a
-electron analogue of an
-electron Kondo insulator and, in addition, a "topological Kondo insulator" (TKI). The overall behavior of the magnetoresistance of FeSi at temperatures above and below the onset temperature
= 19 K of the CSS is similar to that of SmB
. The two energy gaps, inferred from the ρ(
) data in the semiconducting regime, increase with pressure up to about 7 GPa, followed by a drop which coincides with a sharp suppression of
. Several studies of ρ(
) under pressure on SmB
reveal behavior similar to that of FeSi in which the two energy gaps vanish at a critical pressure near the pressure at which
vanishes, although the energy gaps in SmB
initially decrease with pressure, whereas in FeSi they increase with pressure. The MFMMS measurements showed a sharp feature at
≈ 19 K for FeSi, which could be due to ferromagnetic ordering of the CSS. However, no such feature was observed at
≈ 4.5 K for SmB
.</description><identifier>ISSN: 0027-8424</identifier><identifier>EISSN: 1091-6490</identifier><identifier>DOI: 10.1073/pnas.2216367120</identifier><identifier>PMID: 36791111</identifier><language>eng</language><publisher>United States: National Academy of Sciences</publisher><subject>CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS ; conducting surface state ; Critical pressure ; Electrical resistivity ; Energy gap ; Ferromagnetism ; Intermetallic compounds ; Iron silicide ; Kondo insulator ; Magnetic fields ; Magnetic properties ; Magnetoresistance ; Magnetoresistivity ; Microwave radiation ; Microwaves ; Physical Sciences ; Pressure ; pressure-induced metallization ; Samarium compounds ; Spectroscopy ; topological insulator ; Topology</subject><ispartof>Proceedings of the National Academy of Sciences - PNAS, 2023-02, Vol.120 (8), p.e2216367120-e2216367120</ispartof><rights>Copyright National Academy of Sciences Feb 21, 2023</rights><rights>Copyright © 2023 the Author(s). Published by PNAS. 2023</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c448t-98df5f2f7d993131b0925a027e7baaf7bacd0951caa64c1991d7c214ed7bd1973</citedby><cites>FETCH-LOGICAL-c448t-98df5f2f7d993131b0925a027e7baaf7bacd0951caa64c1991d7c214ed7bd1973</cites><orcidid>0000-0001-5960-1378 ; 0000-0001-8501-7538 ; 0000-0003-2725-1689 ; 0000000327251689 ; 0000000185017538 ; 0000000159601378</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC9974408/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC9974408/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,727,780,784,885,27924,27925,53791,53793</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/36791111$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/biblio/1924839$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Breindel, Alexander J</creatorcontrib><creatorcontrib>Deng, Yuhang</creatorcontrib><creatorcontrib>Moir, Camilla M</creatorcontrib><creatorcontrib>Fang, Yuankan</creatorcontrib><creatorcontrib>Ran, Sheng</creatorcontrib><creatorcontrib>Lou, Hongbo</creatorcontrib><creatorcontrib>Li, Shubin</creatorcontrib><creatorcontrib>Zeng, Qiaoshi</creatorcontrib><creatorcontrib>Shu, Lei</creatorcontrib><creatorcontrib>Wolowiec, Christian T</creatorcontrib><creatorcontrib>Schuller, Ivan K</creatorcontrib><creatorcontrib>Rosa, Priscila F S</creatorcontrib><creatorcontrib>Fisk, Zachary</creatorcontrib><creatorcontrib>Singleton, John</creatorcontrib><creatorcontrib>Maple, M Brian</creatorcontrib><creatorcontrib>Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)</creatorcontrib><title>Probing FeSi, a d -electron topological Kondo insulator candidate, with magnetic field, pressure, and microwaves</title><title>Proceedings of the National Academy of Sciences - PNAS</title><addtitle>Proc Natl Acad Sci U S A</addtitle><description>Recently, evidence for a conducting surface state (CSS) below 19 K was reported for the correlated
-electron small gap semiconductor FeSi. In the work reported herein, the CSS and the bulk phase of FeSi were probed via electrical resistivity ρ measurements as a function of temperature
, magnetic field
to 60 T, and pressure
to 7.6 GPa, and by means of a magnetic field-modulated microwave spectroscopy (MFMMS) technique. The properties of FeSi were also compared with those of the Kondo insulator SmB
to address the question of whether FeSi is a
-electron analogue of an
-electron Kondo insulator and, in addition, a "topological Kondo insulator" (TKI). The overall behavior of the magnetoresistance of FeSi at temperatures above and below the onset temperature
= 19 K of the CSS is similar to that of SmB
. The two energy gaps, inferred from the ρ(
) data in the semiconducting regime, increase with pressure up to about 7 GPa, followed by a drop which coincides with a sharp suppression of
. Several studies of ρ(
) under pressure on SmB
reveal behavior similar to that of FeSi in which the two energy gaps vanish at a critical pressure near the pressure at which
vanishes, although the energy gaps in SmB
initially decrease with pressure, whereas in FeSi they increase with pressure. The MFMMS measurements showed a sharp feature at
≈ 19 K for FeSi, which could be due to ferromagnetic ordering of the CSS. However, no such feature was observed at
≈ 4.5 K for SmB
.</description><subject>CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS</subject><subject>conducting surface state</subject><subject>Critical pressure</subject><subject>Electrical resistivity</subject><subject>Energy gap</subject><subject>Ferromagnetism</subject><subject>Intermetallic compounds</subject><subject>Iron silicide</subject><subject>Kondo insulator</subject><subject>Magnetic fields</subject><subject>Magnetic properties</subject><subject>Magnetoresistance</subject><subject>Magnetoresistivity</subject><subject>Microwave radiation</subject><subject>Microwaves</subject><subject>Physical Sciences</subject><subject>Pressure</subject><subject>pressure-induced metallization</subject><subject>Samarium compounds</subject><subject>Spectroscopy</subject><subject>topological insulator</subject><subject>Topology</subject><issn>0027-8424</issn><issn>1091-6490</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNpdkc9vFCEcxYmxsWv17M0Qe_Gw0wLDDsPFxDStNjbRRD2T7wCzS8PACEwb_3vZbK0_OMDh--HBew-hV5ScUSLa8zlAPmOMdm0nKCNP0IoSSZuOS_IUrQhhouk548foec63hBC56ckzdFxpSetaoflLioMLW3xlv7o1BmxwY73VJcWAS5yjj1unweNPMZiIXciLhxIT1hCMM1DsGt-7ssMTbIMtTuPRWW_WeE425yXVcQXx5HSK93Bn8wt0NILP9uXDeYK-X11-u_jY3Hz-cH3x_qbRnPelkb0ZNyMbhZGypS0diGQbqH6sGADGumlT3VAN0HFNpaRGaEa5NWIwVIr2BL076M7LMFmjbSgJvJqTmyD9VBGc-ncS3E5t452SUnBO-irw5iAQc3Eqa1es3ukYQg1HUcl438oKvX14JcUfi81FTS5r6z0EG5esmBCCUCbIHj39D72NSwo1gz0lJe9J31Xq_EDVvHJOdnz8MSVqX7naV67-VF5vvP7b6CP_u-P2F_BxqLA</recordid><startdate>20230221</startdate><enddate>20230221</enddate><creator>Breindel, Alexander J</creator><creator>Deng, Yuhang</creator><creator>Moir, Camilla M</creator><creator>Fang, Yuankan</creator><creator>Ran, Sheng</creator><creator>Lou, Hongbo</creator><creator>Li, Shubin</creator><creator>Zeng, Qiaoshi</creator><creator>Shu, Lei</creator><creator>Wolowiec, Christian T</creator><creator>Schuller, Ivan K</creator><creator>Rosa, Priscila F S</creator><creator>Fisk, Zachary</creator><creator>Singleton, John</creator><creator>Maple, M Brian</creator><general>National Academy of Sciences</general><general>Proceedings of the National Academy of Sciences</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QG</scope><scope>7QL</scope><scope>7QP</scope><scope>7QR</scope><scope>7SN</scope><scope>7SS</scope><scope>7T5</scope><scope>7TK</scope><scope>7TM</scope><scope>7TO</scope><scope>7U9</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>H94</scope><scope>M7N</scope><scope>P64</scope><scope>RC3</scope><scope>7X8</scope><scope>OTOTI</scope><scope>5PM</scope><orcidid>https://orcid.org/0000-0001-5960-1378</orcidid><orcidid>https://orcid.org/0000-0001-8501-7538</orcidid><orcidid>https://orcid.org/0000-0003-2725-1689</orcidid><orcidid>https://orcid.org/0000000327251689</orcidid><orcidid>https://orcid.org/0000000185017538</orcidid><orcidid>https://orcid.org/0000000159601378</orcidid></search><sort><creationdate>20230221</creationdate><title>Probing FeSi, a d -electron topological Kondo insulator candidate, with magnetic field, pressure, and microwaves</title><author>Breindel, Alexander J ; Deng, Yuhang ; Moir, Camilla M ; Fang, Yuankan ; Ran, Sheng ; Lou, Hongbo ; Li, Shubin ; Zeng, Qiaoshi ; Shu, Lei ; Wolowiec, Christian T ; Schuller, Ivan K ; Rosa, Priscila F S ; Fisk, Zachary ; Singleton, John ; Maple, M Brian</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c448t-98df5f2f7d993131b0925a027e7baaf7bacd0951caa64c1991d7c214ed7bd1973</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS</topic><topic>conducting surface state</topic><topic>Critical pressure</topic><topic>Electrical resistivity</topic><topic>Energy gap</topic><topic>Ferromagnetism</topic><topic>Intermetallic compounds</topic><topic>Iron silicide</topic><topic>Kondo insulator</topic><topic>Magnetic fields</topic><topic>Magnetic properties</topic><topic>Magnetoresistance</topic><topic>Magnetoresistivity</topic><topic>Microwave radiation</topic><topic>Microwaves</topic><topic>Physical Sciences</topic><topic>Pressure</topic><topic>pressure-induced metallization</topic><topic>Samarium compounds</topic><topic>Spectroscopy</topic><topic>topological insulator</topic><topic>Topology</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Breindel, Alexander J</creatorcontrib><creatorcontrib>Deng, Yuhang</creatorcontrib><creatorcontrib>Moir, Camilla M</creatorcontrib><creatorcontrib>Fang, Yuankan</creatorcontrib><creatorcontrib>Ran, Sheng</creatorcontrib><creatorcontrib>Lou, Hongbo</creatorcontrib><creatorcontrib>Li, Shubin</creatorcontrib><creatorcontrib>Zeng, Qiaoshi</creatorcontrib><creatorcontrib>Shu, Lei</creatorcontrib><creatorcontrib>Wolowiec, Christian T</creatorcontrib><creatorcontrib>Schuller, Ivan K</creatorcontrib><creatorcontrib>Rosa, Priscila F S</creatorcontrib><creatorcontrib>Fisk, Zachary</creatorcontrib><creatorcontrib>Singleton, John</creatorcontrib><creatorcontrib>Maple, M Brian</creatorcontrib><creatorcontrib>Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Animal Behavior Abstracts</collection><collection>Bacteriology Abstracts (Microbiology B)</collection><collection>Calcium & Calcified Tissue Abstracts</collection><collection>Chemoreception Abstracts</collection><collection>Ecology Abstracts</collection><collection>Entomology Abstracts (Full archive)</collection><collection>Immunology Abstracts</collection><collection>Neurosciences Abstracts</collection><collection>Nucleic Acids Abstracts</collection><collection>Oncogenes and Growth Factors Abstracts</collection><collection>Virology and AIDS Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>AIDS and Cancer Research Abstracts</collection><collection>Algology Mycology and Protozoology Abstracts (Microbiology C)</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Genetics Abstracts</collection><collection>MEDLINE - Academic</collection><collection>OSTI.GOV</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>Proceedings of the National Academy of Sciences - PNAS</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Breindel, Alexander J</au><au>Deng, Yuhang</au><au>Moir, Camilla M</au><au>Fang, Yuankan</au><au>Ran, Sheng</au><au>Lou, Hongbo</au><au>Li, Shubin</au><au>Zeng, Qiaoshi</au><au>Shu, Lei</au><au>Wolowiec, Christian T</au><au>Schuller, Ivan K</au><au>Rosa, Priscila F S</au><au>Fisk, Zachary</au><au>Singleton, John</au><au>Maple, M Brian</au><aucorp>Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Probing FeSi, a d -electron topological Kondo insulator candidate, with magnetic field, pressure, and microwaves</atitle><jtitle>Proceedings of the National Academy of Sciences - PNAS</jtitle><addtitle>Proc Natl Acad Sci U S A</addtitle><date>2023-02-21</date><risdate>2023</risdate><volume>120</volume><issue>8</issue><spage>e2216367120</spage><epage>e2216367120</epage><pages>e2216367120-e2216367120</pages><issn>0027-8424</issn><eissn>1091-6490</eissn><abstract>Recently, evidence for a conducting surface state (CSS) below 19 K was reported for the correlated
-electron small gap semiconductor FeSi. In the work reported herein, the CSS and the bulk phase of FeSi were probed via electrical resistivity ρ measurements as a function of temperature
, magnetic field
to 60 T, and pressure
to 7.6 GPa, and by means of a magnetic field-modulated microwave spectroscopy (MFMMS) technique. The properties of FeSi were also compared with those of the Kondo insulator SmB
to address the question of whether FeSi is a
-electron analogue of an
-electron Kondo insulator and, in addition, a "topological Kondo insulator" (TKI). The overall behavior of the magnetoresistance of FeSi at temperatures above and below the onset temperature
= 19 K of the CSS is similar to that of SmB
. The two energy gaps, inferred from the ρ(
) data in the semiconducting regime, increase with pressure up to about 7 GPa, followed by a drop which coincides with a sharp suppression of
. Several studies of ρ(
) under pressure on SmB
reveal behavior similar to that of FeSi in which the two energy gaps vanish at a critical pressure near the pressure at which
vanishes, although the energy gaps in SmB
initially decrease with pressure, whereas in FeSi they increase with pressure. The MFMMS measurements showed a sharp feature at
≈ 19 K for FeSi, which could be due to ferromagnetic ordering of the CSS. However, no such feature was observed at
≈ 4.5 K for SmB
.</abstract><cop>United States</cop><pub>National Academy of Sciences</pub><pmid>36791111</pmid><doi>10.1073/pnas.2216367120</doi><orcidid>https://orcid.org/0000-0001-5960-1378</orcidid><orcidid>https://orcid.org/0000-0001-8501-7538</orcidid><orcidid>https://orcid.org/0000-0003-2725-1689</orcidid><orcidid>https://orcid.org/0000000327251689</orcidid><orcidid>https://orcid.org/0000000185017538</orcidid><orcidid>https://orcid.org/0000000159601378</orcidid><oa>free_for_read</oa></addata></record> |
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subjects | CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS conducting surface state Critical pressure Electrical resistivity Energy gap Ferromagnetism Intermetallic compounds Iron silicide Kondo insulator Magnetic fields Magnetic properties Magnetoresistance Magnetoresistivity Microwave radiation Microwaves Physical Sciences Pressure pressure-induced metallization Samarium compounds Spectroscopy topological insulator Topology |
title | Probing FeSi, a d -electron topological Kondo insulator candidate, with magnetic field, pressure, and microwaves |
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