Five-Spin Supramolecule for Simulating Quantum Decoherence of Bell States

We report a supramolecule that contains five spins of two different types and with, crucially, two different and predictable interaction energies between the spins. The supramolecule is characterized, and the interaction energies are demonstrated by electron paramagnetic resonance (EPR) spectroscopy...

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Veröffentlicht in:Journal of the American Chemical Society 2022-09, Vol.144 (35), p.16086-16092
Hauptverfasser: Lockyer, Selena J., Chiesa, Alessandro, Brookfield, Adam, Timco, Grigore A., Whitehead, George F. S., McInnes, Eric J. L., Carretta, Stefano, Winpenny, Richard E. P.
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Sprache:eng
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Zusammenfassung:We report a supramolecule that contains five spins of two different types and with, crucially, two different and predictable interaction energies between the spins. The supramolecule is characterized, and the interaction energies are demonstrated by electron paramagnetic resonance (EPR) spectroscopy. Based on the measured parameters, we propose experiments that would allow this designed supramolecule to be used to simulate quantum decoherence in maximally entangled Bell states that could be used in quantum teleportation.
ISSN:0002-7863
1520-5126
1520-5126
DOI:10.1021/jacs.2c06384