Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography
Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driv...
Gespeichert in:
Veröffentlicht in: | Scientific reports 2016-06, Vol.6 (1), p.28392-28392, Article 28392 |
---|---|
Hauptverfasser: | , , , , , , , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | 28392 |
---|---|
container_issue | 1 |
container_start_page | 28392 |
container_title | Scientific reports |
container_volume | 6 |
creator | Song, Xiaohong Lin, Cheng Sheng, Zhihao Liu, Peng Chen, Zhangjin Yang, Weifeng Hu, Shilin Lin, C. D. Chen, Jing |
description | Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driven back and scatters off the ion(the signal wave). The interference hologram of the two waves may be used to extract target information embedded in the
collision process.
Unlike conventional optical holography, however, propagation of the electron wave packet is affected by the Coulomb potential as well as by the laser field. In addition, electrons are emitted over the whole laser pulse duration, thus multiple interferences may occur. In this work, we used a generalized quantum-trajectory Monte Carlo method to investigate the effect of Coulomb potential and the nonadiabatic subcycle ionization on the photoelectron hologram. We showed that photoelectron hologram can be well described only when the effect of nonadiabatic ionization is accounted for and Coulomb potential can be neglected only in the tunnel ionization regime. Our results help paving the way for establishing photoelectron holography for probing spatial and dynamic properties of atoms and molecules. |
doi_str_mv | 10.1038/srep28392 |
format | Article |
fullrecord | <record><control><sourceid>proquest_pubme</sourceid><recordid>TN_cdi_pubmedcentral_primary_oai_pubmedcentral_nih_gov_4916607</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>4105542361</sourcerecordid><originalsourceid>FETCH-LOGICAL-c465t-c355123ea33793b095314f4daf1db90bee4848848c6cd2c248a9c29f0c2eb2b13</originalsourceid><addsrcrecordid>eNplkVtrFDEUx4NYbFn74BeQoC9VmJrbXPIiyOINCn1pn0Mmk5lJyeaMSaZQP31Tti6rhkAOOT_-5_JH6A0ll5Tw7lOKdmEdl-wFOmNE1BXjjL08ik_ReUp3pJyaSUHlK3TKWs4kaekZmm9D1PfWuzDhAEEPTvc6O4MdBPe7RBCwDgPewuph1-MFsg3ZaY_tOFqTsQs45QhhqkZn_YCXGTJYX1LlE8_gYYp6mR9eo5NR-2TPn98Nuv329Wb7o7q6_v5z--WqMqKpc2V4XVPGrea8lbwnsuZUjGLQIx16SXprRSe6ck1jBmaY6LQ0TI7EMNuznvIN-rzXXdZ-ZwdTuo3aqyW6nY4PCrRTf2eCm9UE90pI2jSkLQLv9gKQslPJuGzNbCCEMpKirKtlWfsGXTxXifBrtSmrnUvGeq-DhTUp2krJKGnaJ733_6B3sMZQdqBoR0rBrmCF-rCnTIRULB0PHVOinnxWB58L-_Z4xAP5x9UCfNwDqaTCZONRyf_UHgEi9rOf</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1800738067</pqid></control><display><type>article</type><title>Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography</title><source>DOAJ Directory of Open Access Journals</source><source>Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals</source><source>Springer Nature OA Free Journals</source><source>Nature Free</source><source>PubMed Central</source><source>Alma/SFX Local Collection</source><source>Free Full-Text Journals in Chemistry</source><creator>Song, Xiaohong ; Lin, Cheng ; Sheng, Zhihao ; Liu, Peng ; Chen, Zhangjin ; Yang, Weifeng ; Hu, Shilin ; Lin, C. D. ; Chen, Jing</creator><creatorcontrib>Song, Xiaohong ; Lin, Cheng ; Sheng, Zhihao ; Liu, Peng ; Chen, Zhangjin ; Yang, Weifeng ; Hu, Shilin ; Lin, C. D. ; Chen, Jing ; Shantou Univ., Shantou, Guangdong (China, Peoples Republic of)</creatorcontrib><description>Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driven back and scatters off the ion(the signal wave). The interference hologram of the two waves may be used to extract target information embedded in the
collision process.
Unlike conventional optical holography, however, propagation of the electron wave packet is affected by the Coulomb potential as well as by the laser field. In addition, electrons are emitted over the whole laser pulse duration, thus multiple interferences may occur. In this work, we used a generalized quantum-trajectory Monte Carlo method to investigate the effect of Coulomb potential and the nonadiabatic subcycle ionization on the photoelectron hologram. We showed that photoelectron hologram can be well described only when the effect of nonadiabatic ionization is accounted for and Coulomb potential can be neglected only in the tunnel ionization regime. Our results help paving the way for establishing photoelectron holography for probing spatial and dynamic properties of atoms and molecules.</description><identifier>ISSN: 2045-2322</identifier><identifier>EISSN: 2045-2322</identifier><identifier>DOI: 10.1038/srep28392</identifier><identifier>PMID: 27329071</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/624/400 ; 639/766/36 ; above-threshold-ionization ; Approximation ; ATOMIC AND MOLECULAR PHYSICS ; atoms ; Energy ; Experiments ; Holography ; Humanities and Social Sciences ; induced electron-diffraction ; Ionization ; laser ; Lasers ; Monte Carlo simulation ; multidisciplinary ; phase ; photoionization ; Science ; Simulation</subject><ispartof>Scientific reports, 2016-06, Vol.6 (1), p.28392-28392, Article 28392</ispartof><rights>The Author(s) 2016</rights><rights>Copyright Nature Publishing Group Jun 2016</rights><rights>Copyright © 2016, Macmillan Publishers Limited 2016 Macmillan Publishers Limited</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c465t-c355123ea33793b095314f4daf1db90bee4848848c6cd2c248a9c29f0c2eb2b13</citedby><cites>FETCH-LOGICAL-c465t-c355123ea33793b095314f4daf1db90bee4848848c6cd2c248a9c29f0c2eb2b13</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC4916607/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC4916607/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,723,776,780,860,881,27903,27904,41099,42168,51554,53769,53771</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/27329071$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/servlets/purl/1285910$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Song, Xiaohong</creatorcontrib><creatorcontrib>Lin, Cheng</creatorcontrib><creatorcontrib>Sheng, Zhihao</creatorcontrib><creatorcontrib>Liu, Peng</creatorcontrib><creatorcontrib>Chen, Zhangjin</creatorcontrib><creatorcontrib>Yang, Weifeng</creatorcontrib><creatorcontrib>Hu, Shilin</creatorcontrib><creatorcontrib>Lin, C. D.</creatorcontrib><creatorcontrib>Chen, Jing</creatorcontrib><creatorcontrib>Shantou Univ., Shantou, Guangdong (China, Peoples Republic of)</creatorcontrib><title>Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography</title><title>Scientific reports</title><addtitle>Sci Rep</addtitle><addtitle>Sci Rep</addtitle><description>Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driven back and scatters off the ion(the signal wave). The interference hologram of the two waves may be used to extract target information embedded in the
collision process.
Unlike conventional optical holography, however, propagation of the electron wave packet is affected by the Coulomb potential as well as by the laser field. In addition, electrons are emitted over the whole laser pulse duration, thus multiple interferences may occur. In this work, we used a generalized quantum-trajectory Monte Carlo method to investigate the effect of Coulomb potential and the nonadiabatic subcycle ionization on the photoelectron hologram. We showed that photoelectron hologram can be well described only when the effect of nonadiabatic ionization is accounted for and Coulomb potential can be neglected only in the tunnel ionization regime. Our results help paving the way for establishing photoelectron holography for probing spatial and dynamic properties of atoms and molecules.</description><subject>639/624/400</subject><subject>639/766/36</subject><subject>above-threshold-ionization</subject><subject>Approximation</subject><subject>ATOMIC AND MOLECULAR PHYSICS</subject><subject>atoms</subject><subject>Energy</subject><subject>Experiments</subject><subject>Holography</subject><subject>Humanities and Social Sciences</subject><subject>induced electron-diffraction</subject><subject>Ionization</subject><subject>laser</subject><subject>Lasers</subject><subject>Monte Carlo simulation</subject><subject>multidisciplinary</subject><subject>phase</subject><subject>photoionization</subject><subject>Science</subject><subject>Simulation</subject><issn>2045-2322</issn><issn>2045-2322</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><sourceid>C6C</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNplkVtrFDEUx4NYbFn74BeQoC9VmJrbXPIiyOINCn1pn0Mmk5lJyeaMSaZQP31Tti6rhkAOOT_-5_JH6A0ll5Tw7lOKdmEdl-wFOmNE1BXjjL08ik_ReUp3pJyaSUHlK3TKWs4kaekZmm9D1PfWuzDhAEEPTvc6O4MdBPe7RBCwDgPewuph1-MFsg3ZaY_tOFqTsQs45QhhqkZn_YCXGTJYX1LlE8_gYYp6mR9eo5NR-2TPn98Nuv329Wb7o7q6_v5z--WqMqKpc2V4XVPGrea8lbwnsuZUjGLQIx16SXprRSe6ck1jBmaY6LQ0TI7EMNuznvIN-rzXXdZ-ZwdTuo3aqyW6nY4PCrRTf2eCm9UE90pI2jSkLQLv9gKQslPJuGzNbCCEMpKirKtlWfsGXTxXifBrtSmrnUvGeq-DhTUp2krJKGnaJ733_6B3sMZQdqBoR0rBrmCF-rCnTIRULB0PHVOinnxWB58L-_Z4xAP5x9UCfNwDqaTCZONRyf_UHgEi9rOf</recordid><startdate>20160622</startdate><enddate>20160622</enddate><creator>Song, Xiaohong</creator><creator>Lin, Cheng</creator><creator>Sheng, Zhihao</creator><creator>Liu, Peng</creator><creator>Chen, Zhangjin</creator><creator>Yang, Weifeng</creator><creator>Hu, Shilin</creator><creator>Lin, C. D.</creator><creator>Chen, Jing</creator><general>Nature Publishing Group UK</general><general>Nature Publishing Group</general><scope>C6C</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7X7</scope><scope>7XB</scope><scope>88A</scope><scope>88E</scope><scope>88I</scope><scope>8FE</scope><scope>8FH</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BBNVY</scope><scope>BENPR</scope><scope>BHPHI</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FYUFA</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K9.</scope><scope>LK8</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7P</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>Q9U</scope><scope>7X8</scope><scope>OIOZB</scope><scope>OTOTI</scope><scope>5PM</scope></search><sort><creationdate>20160622</creationdate><title>Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography</title><author>Song, Xiaohong ; Lin, Cheng ; Sheng, Zhihao ; Liu, Peng ; Chen, Zhangjin ; Yang, Weifeng ; Hu, Shilin ; Lin, C. D. ; Chen, Jing</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c465t-c355123ea33793b095314f4daf1db90bee4848848c6cd2c248a9c29f0c2eb2b13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>639/624/400</topic><topic>639/766/36</topic><topic>above-threshold-ionization</topic><topic>Approximation</topic><topic>ATOMIC AND MOLECULAR PHYSICS</topic><topic>atoms</topic><topic>Energy</topic><topic>Experiments</topic><topic>Holography</topic><topic>Humanities and Social Sciences</topic><topic>induced electron-diffraction</topic><topic>Ionization</topic><topic>laser</topic><topic>Lasers</topic><topic>Monte Carlo simulation</topic><topic>multidisciplinary</topic><topic>phase</topic><topic>photoionization</topic><topic>Science</topic><topic>Simulation</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Song, Xiaohong</creatorcontrib><creatorcontrib>Lin, Cheng</creatorcontrib><creatorcontrib>Sheng, Zhihao</creatorcontrib><creatorcontrib>Liu, Peng</creatorcontrib><creatorcontrib>Chen, Zhangjin</creatorcontrib><creatorcontrib>Yang, Weifeng</creatorcontrib><creatorcontrib>Hu, Shilin</creatorcontrib><creatorcontrib>Lin, C. D.</creatorcontrib><creatorcontrib>Chen, Jing</creatorcontrib><creatorcontrib>Shantou Univ., Shantou, Guangdong (China, Peoples Republic of)</creatorcontrib><collection>Springer Nature OA Free Journals</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Health & Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Biology Database (Alumni Edition)</collection><collection>Medical Database (Alumni Edition)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Natural Science Collection</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest One Sustainability</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central Essentials</collection><collection>Biological Science Collection</collection><collection>ProQuest Central</collection><collection>Natural Science Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>Health Research Premium Collection</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>ProQuest Biological Science Collection</collection><collection>Health & Medical Collection (Alumni Edition)</collection><collection>Medical Database</collection><collection>Science Database</collection><collection>Biological Science Database</collection><collection>Publicly Available Content Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central Basic</collection><collection>MEDLINE - Academic</collection><collection>OSTI.GOV - Hybrid</collection><collection>OSTI.GOV</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>Scientific reports</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Song, Xiaohong</au><au>Lin, Cheng</au><au>Sheng, Zhihao</au><au>Liu, Peng</au><au>Chen, Zhangjin</au><au>Yang, Weifeng</au><au>Hu, Shilin</au><au>Lin, C. D.</au><au>Chen, Jing</au><aucorp>Shantou Univ., Shantou, Guangdong (China, Peoples Republic of)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography</atitle><jtitle>Scientific reports</jtitle><stitle>Sci Rep</stitle><addtitle>Sci Rep</addtitle><date>2016-06-22</date><risdate>2016</risdate><volume>6</volume><issue>1</issue><spage>28392</spage><epage>28392</epage><pages>28392-28392</pages><artnum>28392</artnum><issn>2045-2322</issn><eissn>2045-2322</eissn><abstract>Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driven back and scatters off the ion(the signal wave). The interference hologram of the two waves may be used to extract target information embedded in the
collision process.
Unlike conventional optical holography, however, propagation of the electron wave packet is affected by the Coulomb potential as well as by the laser field. In addition, electrons are emitted over the whole laser pulse duration, thus multiple interferences may occur. In this work, we used a generalized quantum-trajectory Monte Carlo method to investigate the effect of Coulomb potential and the nonadiabatic subcycle ionization on the photoelectron hologram. We showed that photoelectron hologram can be well described only when the effect of nonadiabatic ionization is accounted for and Coulomb potential can be neglected only in the tunnel ionization regime. Our results help paving the way for establishing photoelectron holography for probing spatial and dynamic properties of atoms and molecules.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>27329071</pmid><doi>10.1038/srep28392</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record> |
fulltext | fulltext |
identifier | ISSN: 2045-2322 |
ispartof | Scientific reports, 2016-06, Vol.6 (1), p.28392-28392, Article 28392 |
issn | 2045-2322 2045-2322 |
language | eng |
recordid | cdi_pubmedcentral_primary_oai_pubmedcentral_nih_gov_4916607 |
source | DOAJ Directory of Open Access Journals; Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals; Springer Nature OA Free Journals; Nature Free; PubMed Central; Alma/SFX Local Collection; Free Full-Text Journals in Chemistry |
subjects | 639/624/400 639/766/36 above-threshold-ionization Approximation ATOMIC AND MOLECULAR PHYSICS atoms Energy Experiments Holography Humanities and Social Sciences induced electron-diffraction Ionization laser Lasers Monte Carlo simulation multidisciplinary phase photoionization Science Simulation |
title | Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-23T14%3A39%3A49IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_pubme&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Unraveling%20nonadiabatic%20ionization%20and%20Coulomb%20potential%20effect%20in%20strong-field%20photoelectron%20holography&rft.jtitle=Scientific%20reports&rft.au=Song,%20Xiaohong&rft.aucorp=Shantou%20Univ.,%20Shantou,%20Guangdong%20(China,%20Peoples%20Republic%20of)&rft.date=2016-06-22&rft.volume=6&rft.issue=1&rft.spage=28392&rft.epage=28392&rft.pages=28392-28392&rft.artnum=28392&rft.issn=2045-2322&rft.eissn=2045-2322&rft_id=info:doi/10.1038/srep28392&rft_dat=%3Cproquest_pubme%3E4105542361%3C/proquest_pubme%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1800738067&rft_id=info:pmid/27329071&rfr_iscdi=true |