Distilling the Evolving Contributions of Anthropogenic Aerosols and Greenhouse Gases to Large‐Scale Low‐Frequency Surface Ocean Changes Over the Past Century

Anthropogenic aerosols (AER) and greenhouse gases (GHG)—the leading drivers of the forced historical change—produce different large‐scale climate response patterns, with correlations trending from negative to positive over the past century. To understand what caused the time‐evolving comparison between GHG and AER response patterns, we apply a low‐frequency component analysis to historical surface ocean changes from CESM1 single‐forcing large‐ensemble simulations. While GHG response is characterized by its first leading mode, AER response consists of two distinct modes. The first one, featuring long‐term global AER increase and global cooling, opposes GHG response patterns up to the mid‐twentieth century. The second one, featuring multidecadal variations in AER distributions and interhemispheric asymmetric surface ocean changes, appears to reinforce the GHG warming effect over recent decades. AER thus can have both competing and synergistic effects with GHG as their emissions change temporally and spatially. Plain Language Summary Anthropogenically forced climate change over the past century has been mainly caused by two types of emissions: greenhouse gases (GHG) and aerosols (AER). In general, sulfate aerosols from industrial sources can reflect shortwave radiation to yield a cooling effect opposite to the GHG warming effect. However, model simulations isolating GHG and AER forcings show that the large‐scale climate effect of AER does not always dampen the GHG effect. Instead, over recent decades, AER have produced surface ocean response patterns more like the GHG response. Using a novel low‐frequency statistical decomposion, we find that aerosols have driven two distinct modes of climate change patterns over the historical period. The first mode is associated with global aerosol increase, resulting in global‐wide cooling damping the GHG‐induced warming. The second mode is associated with the shift in aerosol emissions from north America/western Europe to southeast Asia, which drives regional changes enhancing the GHG effect. Our results highlight the importance of considering the temporal and spatial evolutions of AER emissions in assessing GHG and AER climate effects and attributing historical anthropogenic climate changes to GHG and AER forcings. Key Points Over the past century, GHG forced response is characterized by a single dominant mode while AER response consists of two distinct modes Monotonic global aerosol increases, mainly from Southeast Asia