Orbital-selective time-domain signature of nematicity dynamics in the charge-density-wave phase of La1.65Eu0.2Sr0.15CuO4
Understanding the interplay between charge, nematic, and structural ordering tendencies in cuprate superconductors is critical to unraveling their complex phase diagram. Using pump–probe time-resolved resonant X-ray scattering on the (0 0 1) Bragg peak at the Cu L3 and O K resonances, we investigate...
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Veröffentlicht in: | Proceedings of the National Academy of Sciences - PNAS 2024-06, Vol.121 (23), p.1 |
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Sprache: | eng |
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Zusammenfassung: | Understanding the interplay between charge, nematic, and structural ordering tendencies in cuprate superconductors is critical to unraveling their complex phase diagram. Using pump–probe time-resolved resonant X-ray scattering on the (0 0 1) Bragg peak at the Cu L3 and O K resonances, we investigate nonequilibrium dynamics of Qa = Qb, = 0 nematic order and its association with both charge density wave (CDW) order and lattice dynamics in La1.65Eu0.2Sr0.15CuO4. The orbital selectivity of the resonant X-ray scattering cross-section allows nematicity dynamics associated with the planar O 2p and Cu 3d states to be distinguished from the response of anisotropic lattice distortions. A direct time-domain comparison of CDW translational-symmetry breaking and nematic rotational-symmetry breaking reveals that these broken symmetries remain closely linked in the photoexcited state, consistent with the stability of CDW topological defects in the investigated pump fluence regime. |
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ISSN: | 0027-8424 1091-6490 1091-6490 |
DOI: | 10.1073/pnas.2400727121 |