Orbital-selective time-domain signature of nematicity dynamics in the charge-density-wave phase of La1.65Eu0.2Sr0.15CuO4

Understanding the interplay between charge, nematic, and structural ordering tendencies in cuprate superconductors is critical to unraveling their complex phase diagram. Using pump–probe time-resolved resonant X-ray scattering on the (0 0 1) Bragg peak at the Cu L3 and O K resonances, we investigate...

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Veröffentlicht in:Proceedings of the National Academy of Sciences - PNAS 2024-06, Vol.121 (23), p.1
Hauptverfasser: Bluschke, Martin, Gupta, Naman K, Jang, Hoyoung, Husain, Ali A, Lee, Byungjune, Kim, Minjune, Na, Mengxing, Dos Remedios, Brandon, Smit, Steef, Moen, Peter, Park, Sang-Youn, Kim, Minseok, Jang, Dogeun, Choi, Hyeongi, Sutarto, Ronny, Reid, Alexander H, Dakovski, Georgi L, Coslovich, Giacomo, Nguyen, Quynh L, Burdet, Nicolas G, Lin, Ming-Fu, Revcolevschi, Alexandre, Park, Jae-Hoon, Geck, Jochen, Turner, Joshua J, Damascelli, Andrea, Hawthorn, David G
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Sprache:eng
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Zusammenfassung:Understanding the interplay between charge, nematic, and structural ordering tendencies in cuprate superconductors is critical to unraveling their complex phase diagram. Using pump–probe time-resolved resonant X-ray scattering on the (0 0 1) Bragg peak at the Cu L3 and O K resonances, we investigate nonequilibrium dynamics of Qa = Qb, = 0 nematic order and its association with both charge density wave (CDW) order and lattice dynamics in La1.65Eu0.2Sr0.15CuO4. The orbital selectivity of the resonant X-ray scattering cross-section allows nematicity dynamics associated with the planar O 2p and Cu 3d states to be distinguished from the response of anisotropic lattice distortions. A direct time-domain comparison of CDW translational-symmetry breaking and nematic rotational-symmetry breaking reveals that these broken symmetries remain closely linked in the photoexcited state, consistent with the stability of CDW topological defects in the investigated pump fluence regime.
ISSN:0027-8424
1091-6490
1091-6490
DOI:10.1073/pnas.2400727121