Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum

We show the first experimental demonstration of room-temperature exciton–polariton (EP) condensation from a bound state in the continuum (BIC). This demonstration is achieved by strongly coupling stable excitons in an organic perylene dye with the extremely long-lived BIC in a dielectric metasurface...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Nano letters 2023-06, Vol.23 (12), p.5603-5609
Hauptverfasser: Berghuis, Anton Matthijs, Castellanos, Gabriel W., Murai, Shunsuke, Pura, Jose Luis, Abujetas, Diego R., van Heijst, Erik, Ramezani, Mohammad, Sánchez-Gil, José A., Rivas, Jaime Gómez
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Beschreibung
Zusammenfassung:We show the first experimental demonstration of room-temperature exciton–polariton (EP) condensation from a bound state in the continuum (BIC). This demonstration is achieved by strongly coupling stable excitons in an organic perylene dye with the extremely long-lived BIC in a dielectric metasurface of silicon nanoparticles. The long lifetime of the BIC, mainly due to the suppression of radiation leakage, allows for EP thermalization to the ground state before decaying. This property results in a condensation threshold of less than 5 μJ cm–2, 1 order of magnitude lower than the lasing threshold reported in similar systems in the weak coupling limit.
ISSN:1530-6984
1530-6992
DOI:10.1021/acs.nanolett.3c01102