Integration of fine-tuned chiral donor with hybrid long/short-range charge-transfer for high-performance circularly polarized electroluminescence

The synergistic integration of a fine-tuned chiral donor with a hybrid long/short-range charge-transfer mechanism offers an accessible pathway to construct highly efficient circularly polarized emitters. Consequently, a notable dissymmetry factor of 1.6 × 10 −3 , concomitantly with a record-setting...

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Veröffentlicht in:Materials horizons 2024-04, Vol.11 (7), p.1752-1759
Hauptverfasser: Yin, Xiaojun, Huang, Haoxin, Li, Nengquan, Li, Wendi, Mo, Xuechao, Huang, Manli, Chen, Guohao, Miao, Jingsheng, Yang, Chuluo
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Sprache:eng
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Zusammenfassung:The synergistic integration of a fine-tuned chiral donor with a hybrid long/short-range charge-transfer mechanism offers an accessible pathway to construct highly efficient circularly polarized emitters. Consequently, a notable dissymmetry factor of 1.6 × 10 −3 , concomitantly with a record-setting maximum external quantum efficiency of 37.4%, is synchronously realized within a single embodiment. Synergistic integration of a fine-tuned chiral donor with hybrid long/short-range charge-transfer offers desirable circularly polarized emitters with both a high dissymmetry factor of 1.6 × 10 −3 and maximum external quantum efficiency of 37.4%.
ISSN:2051-6347
2051-6355
DOI:10.1039/d3mh02146g