Effect of MoS 2 on phenol decomposition in water after high-voltage pulse discharge treatment
Molybdenum disulfide (MoS ) was added to the system after being treated with high-voltage pulse discharge plasma to improve the degradation efficiency of pollutants and reduce energy consumption. The discharge plasma-treated solution contains hydrogen peroxide and metal iron ions, and MoS addition c...
Gespeichert in:
Veröffentlicht in: | Chemosphere (Oxford) 2022-05, Vol.294, p.133808 |
---|---|
Hauptverfasser: | , , , , , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
Zusammenfassung: | Molybdenum disulfide (MoS
) was added to the system after being treated with high-voltage pulse discharge plasma to improve the degradation efficiency of pollutants and reduce energy consumption. The discharge plasma-treated solution contains hydrogen peroxide and metal iron ions, and MoS
addition can cause co-catalytic Fenton reaction. The effects of discharge time, initial pH, phenol concentration, MoS
dosage, discharge voltage, and gas type on phenol removal and aqueous H
O
concentration were mainly investigated. Results showed that the addition of MoS
after plasma treatment can reduce the plasma treatment time by 70% and maintain or even increase the degradation efficiency of phenol from 40% (after 20 min of discharge plasma) to 92% (after turning off the discharge and dosing with MoS
for 30 min). Acidic conditions (pH = 3-4) and oxygen were beneficial to phenol removal. MoS
addition greatly improved the catalytic oxidation of discharge plasma. This study provides a promising direction for water treatment based on plasma technology. |
---|---|
ISSN: | 1879-1298 |
DOI: | 10.1016/j.chemosphere.2022.133808 |