Site regeneration in the Fischer-Tropsch synthesis reaction: a synchronized CO dissociation and C-C coupling pathway

A critical issue in the Fischer-Tropsch synthesis reaction is the blocking of the active sites for low barrier CO dissociation by the C(1) adsorbed species generated from CO dissociation, which can hinder the further steps in the FT process. Here, we propose a synchronized pathway for low barrier CO...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Chemical communications (Cambridge, England) England), 2011-09, Vol.47 (35), p.9822-9824
Hauptverfasser: Shetty, Sharan G, Ciobîcă, Ionel M, Hensen, Emiel J M, van Santen, Rutger A
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Beschreibung
Zusammenfassung:A critical issue in the Fischer-Tropsch synthesis reaction is the blocking of the active sites for low barrier CO dissociation by the C(1) adsorbed species generated from CO dissociation, which can hinder the further steps in the FT process. Here, we propose a synchronized pathway for low barrier CO dissociation and C-C coupling on a corrugated Ru surface.
ISSN:1359-7345
1364-548X
DOI:10.1039/c1cc11499a