Bundling influence on ultrafast optical nonlinearities of single-walled carbon nanotubes in suspension and composite film

Nonlinear optical characteristics of single-walled carbon nanotubes (SWCNTs) dispersed in dichlorobenzene and imbedded in polymer were investigated at 800 nm using the time-resolved optical Kerr gate technique. For systematic study of the influence of SWCNT bundling on optical nonlinearities, SWCNT...

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Veröffentlicht in:Applied physics. B, Lasers and optics Lasers and optics, 2009-09, Vol.97 (1), p.157-162
Hauptverfasser: Lee, H. W., Yim, J. H., Kiran, A. J., Baek, I. H., Lee, S., Yeom, D.-I., Ahn, Y. H., Kim, K., Lee, J., Lim, H., Rotermund, F.
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container_issue 1
container_start_page 157
container_title Applied physics. B, Lasers and optics
container_volume 97
creator Lee, H. W.
Yim, J. H.
Kiran, A. J.
Baek, I. H.
Lee, S.
Yeom, D.-I.
Ahn, Y. H.
Kim, K.
Lee, J.
Lim, H.
Rotermund, F.
description Nonlinear optical characteristics of single-walled carbon nanotubes (SWCNTs) dispersed in dichlorobenzene and imbedded in polymer were investigated at 800 nm using the time-resolved optical Kerr gate technique. For systematic study of the influence of SWCNT bundling on optical nonlinearities, SWCNT solutions with different concentrations and a series of SWCNT/polymer composites deposited on glass substrates with different concentrations and thicknesses were prepared. The nonlinear response was comparable to the pulse duration of the laser used (∼90 fs) both in SWCNT solutions and SWCNT/polymer composites. Over three orders of magnitude enhancement was observed in the third-order nonlinear susceptibility of SWCNT/polymer composite film compared with that of SWCNT solution. An appreciable reduction of microscopic and macroscopic nonlinearities was observed with increasing SWCNT concentrations due to stronger bundling of SWCNTs.
doi_str_mv 10.1007/s00340-009-3532-x
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source Springer Nature - Complete Springer Journals
subjects Bundling
Deposition
Engineering
Exact sciences and technology
Fundamental areas of phenomenology (including applications)
Gates
Lasers
Nonlinear optics
Nonlinearity
Optical Devices
Optical susceptibility, hyperpolarizability
Optics
Photonics
Physical Chemistry
Physics
Physics and Astronomy
Polymer matrix composites
Pulse duration
Quantum Optics
Single wall carbon nanotubes
Ultrafast processes
optical pulse generation and pulse compression
title Bundling influence on ultrafast optical nonlinearities of single-walled carbon nanotubes in suspension and composite film
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