Bundling influence on ultrafast optical nonlinearities of single-walled carbon nanotubes in suspension and composite film
Nonlinear optical characteristics of single-walled carbon nanotubes (SWCNTs) dispersed in dichlorobenzene and imbedded in polymer were investigated at 800 nm using the time-resolved optical Kerr gate technique. For systematic study of the influence of SWCNT bundling on optical nonlinearities, SWCNT...
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Veröffentlicht in: | Applied physics. B, Lasers and optics Lasers and optics, 2009-09, Vol.97 (1), p.157-162 |
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creator | Lee, H. W. Yim, J. H. Kiran, A. J. Baek, I. H. Lee, S. Yeom, D.-I. Ahn, Y. H. Kim, K. Lee, J. Lim, H. Rotermund, F. |
description | Nonlinear optical characteristics of single-walled carbon nanotubes (SWCNTs) dispersed in dichlorobenzene and imbedded in polymer were investigated at 800 nm using the time-resolved optical Kerr gate technique. For systematic study of the influence of SWCNT bundling on optical nonlinearities, SWCNT solutions with different concentrations and a series of SWCNT/polymer composites deposited on glass substrates with different concentrations and thicknesses were prepared. The nonlinear response was comparable to the pulse duration of the laser used (∼90 fs) both in SWCNT solutions and SWCNT/polymer composites. Over three orders of magnitude enhancement was observed in the third-order nonlinear susceptibility of SWCNT/polymer composite film compared with that of SWCNT solution. An appreciable reduction of microscopic and macroscopic nonlinearities was observed with increasing SWCNT concentrations due to stronger bundling of SWCNTs. |
doi_str_mv | 10.1007/s00340-009-3532-x |
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W. ; Yim, J. H. ; Kiran, A. J. ; Baek, I. H. ; Lee, S. ; Yeom, D.-I. ; Ahn, Y. H. ; Kim, K. ; Lee, J. ; Lim, H. ; Rotermund, F.</creator><creatorcontrib>Lee, H. W. ; Yim, J. H. ; Kiran, A. J. ; Baek, I. H. ; Lee, S. ; Yeom, D.-I. ; Ahn, Y. H. ; Kim, K. ; Lee, J. ; Lim, H. ; Rotermund, F.</creatorcontrib><description>Nonlinear optical characteristics of single-walled carbon nanotubes (SWCNTs) dispersed in dichlorobenzene and imbedded in polymer were investigated at 800 nm using the time-resolved optical Kerr gate technique. For systematic study of the influence of SWCNT bundling on optical nonlinearities, SWCNT solutions with different concentrations and a series of SWCNT/polymer composites deposited on glass substrates with different concentrations and thicknesses were prepared. The nonlinear response was comparable to the pulse duration of the laser used (∼90 fs) both in SWCNT solutions and SWCNT/polymer composites. Over three orders of magnitude enhancement was observed in the third-order nonlinear susceptibility of SWCNT/polymer composite film compared with that of SWCNT solution. 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W.</creatorcontrib><creatorcontrib>Yim, J. H.</creatorcontrib><creatorcontrib>Kiran, A. J.</creatorcontrib><creatorcontrib>Baek, I. H.</creatorcontrib><creatorcontrib>Lee, S.</creatorcontrib><creatorcontrib>Yeom, D.-I.</creatorcontrib><creatorcontrib>Ahn, Y. H.</creatorcontrib><creatorcontrib>Kim, K.</creatorcontrib><creatorcontrib>Lee, J.</creatorcontrib><creatorcontrib>Lim, H.</creatorcontrib><creatorcontrib>Rotermund, F.</creatorcontrib><title>Bundling influence on ultrafast optical nonlinearities of single-walled carbon nanotubes in suspension and composite film</title><title>Applied physics. B, Lasers and optics</title><addtitle>Appl. Phys. B</addtitle><description>Nonlinear optical characteristics of single-walled carbon nanotubes (SWCNTs) dispersed in dichlorobenzene and imbedded in polymer were investigated at 800 nm using the time-resolved optical Kerr gate technique. For systematic study of the influence of SWCNT bundling on optical nonlinearities, SWCNT solutions with different concentrations and a series of SWCNT/polymer composites deposited on glass substrates with different concentrations and thicknesses were prepared. The nonlinear response was comparable to the pulse duration of the laser used (∼90 fs) both in SWCNT solutions and SWCNT/polymer composites. Over three orders of magnitude enhancement was observed in the third-order nonlinear susceptibility of SWCNT/polymer composite film compared with that of SWCNT solution. An appreciable reduction of microscopic and macroscopic nonlinearities was observed with increasing SWCNT concentrations due to stronger bundling of SWCNTs.</description><subject>Bundling</subject><subject>Deposition</subject><subject>Engineering</subject><subject>Exact sciences and technology</subject><subject>Fundamental areas of phenomenology (including applications)</subject><subject>Gates</subject><subject>Lasers</subject><subject>Nonlinear optics</subject><subject>Nonlinearity</subject><subject>Optical Devices</subject><subject>Optical susceptibility, hyperpolarizability</subject><subject>Optics</subject><subject>Photonics</subject><subject>Physical Chemistry</subject><subject>Physics</subject><subject>Physics and Astronomy</subject><subject>Polymer matrix composites</subject><subject>Pulse duration</subject><subject>Quantum Optics</subject><subject>Single wall carbon nanotubes</subject><subject>Ultrafast processes; optical pulse generation and pulse compression</subject><issn>0946-2171</issn><issn>1432-0649</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2009</creationdate><recordtype>article</recordtype><recordid>eNp9kctKBDEQRYMoOD4-wF1vxFVr0q90liq-QHCj61CTrkgkk7SpblT8mfkWv8zIiEuzSUjOvVAnjB0Jfio4l2fEed3wknNV1m1dle9bbCGafOBdo7bZgqumKyshxS7bI3rheXV9v2CfF3MYvAvPhQvWzxgMFjEUs58SWKCpiOPkDPgixJAxhOQmh1RE-7WmHPNYvoH3OBQG0jInA4Q4zcuMuFDQTCMGcvkeQkbiaozkJvxaW-dXB2zHgic8_N332dP11ePlbXn_cHN3eX5fmrrlU6m6YVDCWMmB9_3Q99AZ2YklwmAlKCFUK6VsexxshXUlajWgtbLpYKkqo7DeZyeb3jHF1xlp0itHBr2HgHEmrYRSjZKyyqTYkCZFooRWj8mtIH1owfWPZ73xrLNn_eNZv-fM8W87UBZlEwTj6C9YCZW_QbWZqzYc5afwjEm_xDmFPPg_5d-QUZMm</recordid><startdate>20090901</startdate><enddate>20090901</enddate><creator>Lee, H. W.</creator><creator>Yim, J. H.</creator><creator>Kiran, A. J.</creator><creator>Baek, I. H.</creator><creator>Lee, S.</creator><creator>Yeom, D.-I.</creator><creator>Ahn, Y. H.</creator><creator>Kim, K.</creator><creator>Lee, J.</creator><creator>Lim, H.</creator><creator>Rotermund, F.</creator><general>Springer-Verlag</general><general>Springer</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>20090901</creationdate><title>Bundling influence on ultrafast optical nonlinearities of single-walled carbon nanotubes in suspension and composite film</title><author>Lee, H. W. ; Yim, J. H. ; Kiran, A. J. ; Baek, I. H. ; Lee, S. ; Yeom, D.-I. ; Ahn, Y. 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W.</creatorcontrib><creatorcontrib>Yim, J. H.</creatorcontrib><creatorcontrib>Kiran, A. J.</creatorcontrib><creatorcontrib>Baek, I. H.</creatorcontrib><creatorcontrib>Lee, S.</creatorcontrib><creatorcontrib>Yeom, D.-I.</creatorcontrib><creatorcontrib>Ahn, Y. H.</creatorcontrib><creatorcontrib>Kim, K.</creatorcontrib><creatorcontrib>Lee, J.</creatorcontrib><creatorcontrib>Lim, H.</creatorcontrib><creatorcontrib>Rotermund, F.</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied physics. B, Lasers and optics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lee, H. W.</au><au>Yim, J. H.</au><au>Kiran, A. J.</au><au>Baek, I. H.</au><au>Lee, S.</au><au>Yeom, D.-I.</au><au>Ahn, Y. H.</au><au>Kim, K.</au><au>Lee, J.</au><au>Lim, H.</au><au>Rotermund, F.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Bundling influence on ultrafast optical nonlinearities of single-walled carbon nanotubes in suspension and composite film</atitle><jtitle>Applied physics. B, Lasers and optics</jtitle><stitle>Appl. Phys. B</stitle><date>2009-09-01</date><risdate>2009</risdate><volume>97</volume><issue>1</issue><spage>157</spage><epage>162</epage><pages>157-162</pages><issn>0946-2171</issn><eissn>1432-0649</eissn><abstract>Nonlinear optical characteristics of single-walled carbon nanotubes (SWCNTs) dispersed in dichlorobenzene and imbedded in polymer were investigated at 800 nm using the time-resolved optical Kerr gate technique. For systematic study of the influence of SWCNT bundling on optical nonlinearities, SWCNT solutions with different concentrations and a series of SWCNT/polymer composites deposited on glass substrates with different concentrations and thicknesses were prepared. The nonlinear response was comparable to the pulse duration of the laser used (∼90 fs) both in SWCNT solutions and SWCNT/polymer composites. Over three orders of magnitude enhancement was observed in the third-order nonlinear susceptibility of SWCNT/polymer composite film compared with that of SWCNT solution. An appreciable reduction of microscopic and macroscopic nonlinearities was observed with increasing SWCNT concentrations due to stronger bundling of SWCNTs.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer-Verlag</pub><doi>10.1007/s00340-009-3532-x</doi><tpages>6</tpages></addata></record> |
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subjects | Bundling Deposition Engineering Exact sciences and technology Fundamental areas of phenomenology (including applications) Gates Lasers Nonlinear optics Nonlinearity Optical Devices Optical susceptibility, hyperpolarizability Optics Photonics Physical Chemistry Physics Physics and Astronomy Polymer matrix composites Pulse duration Quantum Optics Single wall carbon nanotubes Ultrafast processes optical pulse generation and pulse compression |
title | Bundling influence on ultrafast optical nonlinearities of single-walled carbon nanotubes in suspension and composite film |
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