Innovative membrane based process for the selective oxidation of light alkanes assisted by the Fenton system

Innovative membrane based process for the selective oxidation of light alkanes assisted by the Fenton system

Selective oxidation of light alkanes under mild conditions (temp, 80–120 °C; pressure, 140 kPa) mediated by Fe2+/H2O2 Fenton system on Nafion based composite membranes is studied in a multifunctional three phase catalytic membrane reactor (3PCMR). The role of textural properties and acid functionali...

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Veröffentlicht in:Asia-Pacific journal of chemical engineering 2010-01, Vol.5 (1), p.66-72
Hauptverfasser: Espro, C., Mendolia, F., Marini, S., Frusteri, F., Parmaliana, A.
Format: Artikel
Sprache:eng
Schlagworte:
light alkanes selective oxidation
membrane reactor
oxygenated products
superacid membranes
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Zusammenfassung:Selective oxidation of light alkanes under mild conditions (temp, 80–120 °C; pressure, 140 kPa) mediated by Fe2+/H2O2 Fenton system on Nafion based composite membranes is studied in a multifunctional three phase catalytic membrane reactor (3PCMR). The role of textural properties and acid functionality on the catalytic performance of the Nafion composite membranes is outlined. The features of the multifunctional 3PCMR, enabling reaction along with product separation and recovery, are discussed. Copyright © 2009 Curtin University of Technology and John Wiley & Sons, Ltd.
ISSN:1932-2135
1932-2143
DOI:10.1002/apj.390