Unified ab initio treatment of attosecond photoionization and Compton scattering
We present a new theoretical approach to attosecond laser-assisted photo- and Compton ionization. Attosecond x-ray absorption and scattering are described by -matrices, which are coherent superpositions of 'monochromatic' -matrices in a laser-modified Furry representation. Besides refining...
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Veröffentlicht in: | Journal of physics. B, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2009-10, Vol.42 (20), p.205601-205601 (8) |
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Format: | Artikel |
Sprache: | eng |
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Zusammenfassung: | We present a new theoretical approach to attosecond laser-assisted photo- and Compton ionization. Attosecond x-ray absorption and scattering are described by -matrices, which are coherent superpositions of 'monochromatic' -matrices in a laser-modified Furry representation. Besides refining the existing theory of the soft x-ray photoelectron attosecond streak camera and spectral phase interferometry (ASC and ASPI), we formulate a theory of hard x-ray photoelectron and Compton ASC and ASPI. The resulting scheme has a simple structure and leads to closed-form expressions for ionization amplitudes. We investigate Compton electron interference in the separable Coulomb-Volkov continuum with both Coulomb and laser fields treated non-perturbatively. We find that at laser-field intensities below 1013 Wcm-2 normalized Compton lines almost coincide with the lines obtained in the laser-free regime. At higher intensities, attosecond interferences survive integration over electron momenta, and feature prominently in the Compton lines themselves. We define a regime where the electron ground-state density can be measured with controllable accuracy in an attosecond time interval. The new theory provides a firm basis for extracting photo- and Compton electron phases and atomic and molecular wavefunctions from experimental data. |
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ISSN: | 0953-4075 1361-6455 |
DOI: | 10.1088/0953-4075/42/20/205601 |