A Mesoporous Template Route to the Low-Temperature Preparation of Efficient Green Light Emitting Zn2SiO4:Mn Phosphors

Green light emitting Zn2SiO4:Mn phosphors have been prepared via a low-temperature solid-state reaction using mesoporous silica SBA-15 template. This mesoporous silica template method features low-temperature formation of phosphors and easy doping. The structure and morphology of the phosphors were...

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Veröffentlicht in:The journal of physical chemistry. B 2005-01, Vol.109 (2), p.731-735
Hauptverfasser: Xiong, Liangming, Shi, Jianlin, Gu, Jinlou, Li, Liang, Huang, Weimin, Gao, Jianhua, Ruan, Meiling
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Sprache:eng
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Zusammenfassung:Green light emitting Zn2SiO4:Mn phosphors have been prepared via a low-temperature solid-state reaction using mesoporous silica SBA-15 template. This mesoporous silica template method features low-temperature formation of phosphors and easy doping. The structure and morphology of the phosphors were characterized by XRD, SEM, TEM, and N2 adsorption/desorption techniques, which confirmed the single crystallinity, ordered mesostructure, closed pore channels, and elongated ropelike morphology. The luminescent properties were examined by photoluminescence spectroscopy at room temperature, and the results of fluorescence decay time measurements show non-single-exponential decay behavior and a decrease of the decay time with an increase of the Mn concentration.
ISSN:1520-6106
1520-5207
DOI:10.1021/jp045630s