Spin thermal conductivity of the haldane chain compound Y(2)BaNiO(5)

We have measured the thermal conductivity of the spin S=1 chain compound Y(2)BaNiO(5). Analyzing the anisotropy of the thermal transport allows us to identify a definite spin-mediated thermal conductivity kappa(s) along the chain direction. The calculated spin-related energy diffusion constant D(E)(...

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Veröffentlicht in:Physical review letters 2006-09, Vol.97 (11), p.115901-115901
Hauptverfasser: Kordonis, K, Sologubenko, A V, Lorenz, T, Cheong, S-W, Freimuth, A
Format: Artikel
Sprache:eng
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Zusammenfassung:We have measured the thermal conductivity of the spin S=1 chain compound Y(2)BaNiO(5). Analyzing the anisotropy of the thermal transport allows us to identify a definite spin-mediated thermal conductivity kappa(s) along the chain direction. The calculated spin-related energy diffusion constant D(E)(T) shows a broad peak around 120 K. Close to room temperature, D(E)(T) approaches the theoretically predicted high-temperature value, while scattering of spin excitations by magnetic impurities seems to be the major limiting factor of kappa(s) at low temperature.
ISSN:0031-9007