Triple-Resonance Coherent Anti-Stokes Raman Scattering Microspectroscopy

Fluorescence‐free microscopy: A new nonlinear optical microspectroscopy technique, femtosecond (fs) triple‐resonance coherent anti‐Stokes Raman scattering, in which the amplitude and phase of input fs laser pulses are optimally shaped to be in triple resonance with the molecular electronic and vibra...

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Veröffentlicht in:Chemphyschem 2009-02, Vol.10 (2), p.344-347
Hauptverfasser: Min, Wei, Lu, Sijia, Holtom, Gary R., Xie, X. Sunney
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creator Min, Wei
Lu, Sijia
Holtom, Gary R.
Xie, X. Sunney
description Fluorescence‐free microscopy: A new nonlinear optical microspectroscopy technique, femtosecond (fs) triple‐resonance coherent anti‐Stokes Raman scattering, in which the amplitude and phase of input fs laser pulses are optimally shaped to be in triple resonance with the molecular electronic and vibrational transitions, generates a coherent nonlinear signal beam at a new color with a highest possible efficiency (see figure). Fluorescence‐free microscopy: A new nonlinear optical microspectroscopy technique, femtosecond (fs) triple‐resonance coherent anti‐Stokes Raman scattering, in which the amplitude and phase of input fs laser pulses are optimally shaped to be in triple resonance with the molecular electronic and vibrational transitions, generates a coherent nonlinear signal beam at a new color with a highest possible efficiency (see figure).
doi_str_mv 10.1002/cphc.200800502
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source Wiley Online Library Journals Frontfile Complete
subjects Atomic and molecular physics
CARS microscopy
Exact sciences and technology
fluorescence-free microscopy techniques
Molecular properties and interactions with photons
Molecular spectra
nonlinear optics
Physics
Raman and rayleigh spectra (including optical scattering)
resonance Raman scattering
vibrational coherence
title Triple-Resonance Coherent Anti-Stokes Raman Scattering Microspectroscopy
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