The Electron-Transfer Rate Processes In Biological Systems

The Electron-Transfer Rate Processes In Biological Systems

The reaction coordinates for the electron transfer (ET) reactions are discussed. The channel-based reaction-diffusion equations are solved analytically for two biological electron transfer models, which allow us build an ET rate constant which modifies the Marcus-Jortner formula by adding a dynamic...

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Hauptverfasser: Zhu, Jianjun, Bai, Tong-Chun, Wei, Dongqing
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description The reaction coordinates for the electron transfer (ET) reactions are discussed. The channel-based reaction-diffusion equations are solved analytically for two biological electron transfer models, which allow us build an ET rate constant which modifies the Marcus-Jortner formula by adding a dynamic correction factor. The dynamic correction factor can reduce the ET rate by orders of magnitude. The theory has been compared with experiment with fairly good result.
doi_str_mv 10.1063/1.3108381
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title The Electron-Transfer Rate Processes In Biological Systems
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