Topologically Engineered High‑Q Quasi-BIC Metasurfaces for Enhanced Near-Infrared Emission in PbS Quantum Dots

Enhancing photoluminescence (PL) efficiency in colloidal quantum dots is pivotal for next-generation near-infrared photodetectors, imaging systems, and photonic devices. Conventional methods, especially metal-based plasmonic structures, suffer from large optical losses, which limits their practical...

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Veröffentlicht in:Nano letters 2025-01, Vol.25 (6), p.2357-2365
Hauptverfasser: Guo, Jiaoyang, Jin, Rong, Fu, Zhenchu, Zhang, Yukang, Yu, Feilong, Chen, Jin, Wang, Xingjun, Huang, Lujun, Zhou, Chaobiao, Chen, Xiaoshuang, Lu, Wei, Li, Guanhai
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Sprache:eng
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Zusammenfassung:Enhancing photoluminescence (PL) efficiency in colloidal quantum dots is pivotal for next-generation near-infrared photodetectors, imaging systems, and photonic devices. Conventional methods, especially metal-based plasmonic structures, suffer from large optical losses, which limits their practical use. Here, we introduce a quasi-bound state in the continuum (quasi-BIC) metasurface on a silicon-on-insulator platform, tailored to provide high-quality factor resonances with minimized losses. Utilizing topological charge engineering and controlled in-plane asymmetry in silicon cylinder arrays, we developed a robust quasi-BIC capable of maintaining a high Q factor across a broad angular range, achieving an experimental Q factor of 3031 at normal incidence. This approach significantly enhances near-field interactions, achieving a ≤110-fold increase in PL for PbS quantum dots at 33 K and a 41-fold enhancement at room temperature. Our findings offer a scalable, cost-effective solution for enhancing light emission in advanced optoelectronic applications.
ISSN:1530-6984
1530-6992
1530-6992
DOI:10.1021/acs.nanolett.4c05710