Highly Elastic, Fatigue-Resistant, and Antifreezing MXene Functionalized Organohydrogels as Flexible Pressure Sensors for Human Motion Monitoring

Conductive organohydrogels-based flexible pressure sensors have gained considerable attention in health monitoring, artificial skin, and human-computer interaction due to their excellent biocompatibility, wearability, and versatility. However, hydrogels’ unsatisfactory mechanical and unstable electrical properties hinder their comprehensive application. Herein, an elastic, fatigue-resistant, and antifreezing poly­(vinyl alcohol) (PVA)/lipoic acid (LA) organohydrogel with a double-network structure and reversible cross-linking interactions has been designed, and MXene as a conductive filler is functionalized into organohydrogel to further enhance the diverse sensing performance of flexible pressure sensors. The as-fabricated MXene-based PVA/LA organohydrogels (PLBM) exhibit stable fatigue resistance for over 450 cycles under 40% compressive strain, excellent elasticity, antifreezing properties (