Fermi Surface Nesting Driving the RKKY Interaction in the Centrosymmetric Skyrmion Magnet Gd_{2}PdSi_{3}

The magnetic skyrmions generated in a centrosymmetric crystal were recently first discovered in Gd_{2}PdSi_{3}. In light of this, we observe the electronic structure by angle-resolved photoemission spectroscopy and unveil its direct relationship with the magnetism in this compound. The Fermi surface...

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Veröffentlicht in:Physical review letters 2024-07, Vol.133 (1), p.016401
Hauptverfasser: Dong, Yuyang, Arai, Yosuke, Kuroda, Kenta, Ochi, Masayuki, Tanaka, Natsumi, Wan, Yuxuan, Watson, Matthew D, Kim, Timur K, Cacho, Cephise, Hashimoto, Makoto, Lu, Donghui, Aoki, Yuji, Matsuda, Tatsuma D, Kondo, Takeshi
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Sprache:eng
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Zusammenfassung:The magnetic skyrmions generated in a centrosymmetric crystal were recently first discovered in Gd_{2}PdSi_{3}. In light of this, we observe the electronic structure by angle-resolved photoemission spectroscopy and unveil its direct relationship with the magnetism in this compound. The Fermi surface and band dispersions are demonstrated to have a good agreement with the density functional theory calculations carried out with careful consideration of the crystal superstructure. Most importantly, we find that the three-dimensional Fermi surface has extended nesting which matches well the q vector of the magnetic order detected by recent scattering measurements. The consistency we find among angle-resolved photoemission spectroscopy, density functional theory, and the scattering measurements suggests the Ruderman-Kittel-Kasuya-Yosida interaction involving itinerant electrons to be the formation mechanism of skyrmions in Gd_{2}PdSi_{3}.
ISSN:1079-7114
1079-7114
DOI:10.1103/PhysRevLett.133.016401