Tuning the Flat Band in Bi2O2Se by Pressure to Induce Superconductivity

The discovery of superconductivity in twisted bilayer graphene has reignited enthusiasm in the field of flat-band superconductivity. However, important challenges remain, such as constructing a flat-band structure and inducing a superconducting state in materials. Here, we successfully achieved supe...

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Veröffentlicht in:Journal of the American Chemical Society 2024-03, Vol.146 (11), p.7324-7331
Hauptverfasser: Tian, Hui, Tu, Teng, Jin, Xilian, Li, Chenyi, Lin, Tao, Dong, Qing, Jing, Xiaoling, Liu, Bo, Liu, Ran, Li, Da, Liu, Zhongkai, Li, Quanjun, Peng, Hailin, Liu, Bingbing
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Sprache:eng
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Zusammenfassung:The discovery of superconductivity in twisted bilayer graphene has reignited enthusiasm in the field of flat-band superconductivity. However, important challenges remain, such as constructing a flat-band structure and inducing a superconducting state in materials. Here, we successfully achieved superconductivity in Bi2O2Se by pressure-tuning the flat-band electronic structure. Experimental measurements combined with theoretical calculations reveal that the occurrence of pressure-induced superconductivity at 30 GPa is associated with a flat-band electronic structure near the Fermi level. Moreover, in Bi2O2Se, a van Hove singularity is observed at the Fermi level alongside pronounced Fermi surface nesting. These remarkable features play a crucial role in promoting strong electron–phonon interactions, thus potentially enhancing the superconducting properties of the material. These findings demonstrate that pressure offers a potential experimental strategy for precisely tuning the flat band and achieving superconductivity.
ISSN:0002-7863
1520-5126
DOI:10.1021/jacs.3c11984