Novel soy protein isolate/sodium alginate-based functional aerogel for efficient uptake of organic dye from effluents

In response to the increasing global concern regarding water pollution, there is a growing demand for the development of novel adsorbents capable of effectively eliminating hazardous organic pollutants from effluents. In this study, we present a functional soy protein isolate (SPI)/sodium alginate (ALG)/polyethyleneimine (PEI) aerogel prepared via a facile chemical crosslinking process as a novel adsorbent with excellent capabilities for removing toxic methyl blue (MB) dye from effluents. Thanks to the synergistic dense oxygen and nitrogen-containing functional groups in the networks, the ALG/SPI/PEI (ASP) aerogel displayed high adsorption capacity for MB (106.3 mg/g) complying the adsorption kinetics and isotherm with the pseudo-second-order and Langmuir models, respectively. Remarkably, the MB adsorption capability of the ASP aerogel surpasses that of its pristine counterpart and outperforms recently reported adsorbents. Moreover, the aerogel maintained >80% of initial adsorption capability in the fourth regenerative cycle, indicating excellent reusability. The superior MB adsorbability coupled with high-efficiency regenerability in this study reveal the significant potential of ASP aerogel in efficiently eliminating organic dye from wastewater. [Display omitted] •Novel ALG/SPI/PEI aerogel with superior dye coordination property was developed.•The aerogel revealed superior methyl blue (MB) dye uptake property in effluents.•PEI modification enabled immense active sites, porosity, eventually enhanced MB uptake.•Adsorption mechanism involves chelation between the active sites of aerogel and MB.