A Lotus Seedpods‐Inspired Interfacial Solar Steam Generator with Outstanding Salt Tolerance and Mechanical Properties for Efficient and Stable Seawater Desalination

Interfacial solar steam generators (ISSGs) can capture solar energy and concentrate the heat at the gas–liquid interface, resulting in efficient water evaporation. However, traditional ISSGs have limitations in long‐term seawater desalination processes, such as limited light absorption area, slow wa...

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Veröffentlicht in:Small (Weinheim an der Bergstrasse, Germany) Germany), 2023-12, Vol.19 (52), p.e2304877-n/a
Hauptverfasser: Ma, Haodong, Yu, Lingjie, Li, Zhenzhen, Chen, Jianglong, Meng, Jiaguang, Song, Qingwen, Liu, Yaming, Wang, Yongzhen, Wu, Qian, Miao, Menghe, Zhi, Chao
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Sprache:eng
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Zusammenfassung:Interfacial solar steam generators (ISSGs) can capture solar energy and concentrate the heat at the gas–liquid interface, resulting in efficient water evaporation. However, traditional ISSGs have limitations in long‐term seawater desalination processes, such as limited light absorption area, slow water transport speed, severe surface salt accumulation, and weak mechanical performance. Inspired by lotus seedpods, a novel ISSG (rGO‐SA‐PSF) is developed by treating a 3D warp‐knitted spacer fabric with plasma (PSF) and combining it with sodium alginate (SA) and reduces graphene oxide (rGO). The rGO‐SA‐PSF utilizes a core‐suction effect to achieve rapid water pumping and employs aerogel to encapsulate the plasma‐treated spacer yarns to create the lotus seedpod‐inspired hydrophilic stems, innovatively constructing multiple directional water transport channels. Simultaneously, the large holes of rGO‐SA‐PSF on the upper layer form lotus seedpod‐inspired head concave holes, enabling efficient light capture. Under 1 kW m−2 illumination, rGO‐SA‐PSF exhibits a rapid evaporation rate of 1.85 kg m−2 h−1, with an efficiency of 96.4%. Additionally, it shows superior salt tolerance (with no salt accumulation during continuous evaporation for 10 h in 10% brine) and self‐desalination performance during long‐term seawater desalination processes. This biomimetic ISSG offers a promising solution for efficient and stable seawater desalination and wastewater purification. Inspired by lotus seedpods, an interfacial solar steam generator is developed combining 3D warp‐knitted spacer fabric with reduced graphene oxide (rGO) and sodium alginate. It achieves efficient water pumping through core‐suction, water transportation via directional channels, and light capturing via concave holes. It exhibits 1.85 kg m−2 h−1 rate and 96.4% efficiency under 1 kW m−2, surpassing most rGO‐based generators.
ISSN:1613-6810
1613-6829
DOI:10.1002/smll.202304877