Ultrafast exciton fluid flow in an atomically thin MoS2 semiconductor
Excitons (coupled electron–hole pairs) in semiconductors can form collective states that sometimes exhibit spectacular nonlinear properties. Here, we show experimental evidence of a collective state of short-lived excitons in a direct-bandgap, atomically thin MoS 2 semiconductor whose propagation re...
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Veröffentlicht in: | Nature nanotechnology 2023-09, Vol.18 (9), p.1012-1019 |
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Sprache: | eng |
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Zusammenfassung: | Excitons (coupled electron–hole pairs) in semiconductors can form collective states that sometimes exhibit spectacular nonlinear properties. Here, we show experimental evidence of a collective state of short-lived excitons in a direct-bandgap, atomically thin MoS
2
semiconductor whose propagation resembles that of a classical liquid as suggested by the nearly uniform photoluminescence through the MoS
2
monolayer regardless of crystallographic defects and geometric constraints. The exciton fluid flows over ultralong distances (at least 60 μm) at a speed of ~1.8 × 10
7
m s
−1
(~6% the speed of light). The collective phase emerges above a critical laser power, in the absence of free charges and below a critical temperature (usually
T
c
≈ 150 K) approaching room temperature in hexagonal-boron-nitride-encapsulated devices. Our theoretical simulations suggest that momentum is conserved and local equilibrium is achieved among excitons; both these features are compatible with a fluid dynamics description of the exciton transport.
Evidence is provided for the formation of a collective state of short-lived excitons whose propagation resembles that of a classical liquid flows, with a speed reaching ~6% the speed of light. |
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ISSN: | 1748-3387 1748-3395 1748-3395 |
DOI: | 10.1038/s41565-023-01438-8 |