Highly Localized Optical Field Enhancement at Neon Ion Sputtered Tungsten Nanotips

We present laser-driven rescattering of electrons at a nanometric protrusion (nanotip), which is fabricated with an in situ neon ion sputtering technique applied to a tungsten needle tip. Electron energy spectra obtained before and after the sputtering show rescattering features, such as a plateau a...

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Veröffentlicht in:Nano letters 2023-08, Vol.23 (15), p.7114-7119
Hauptverfasser: Paschen, Timo, Brückner, Leon, Wu, Mingjian, Spiecker, Erdmann, Hommelhoff, Peter
Format: Artikel
Sprache:eng
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Zusammenfassung:We present laser-driven rescattering of electrons at a nanometric protrusion (nanotip), which is fabricated with an in situ neon ion sputtering technique applied to a tungsten needle tip. Electron energy spectra obtained before and after the sputtering show rescattering features, such as a plateau and high-energy cutoff. Extracting the optical near-field enhancement in both cases, we observe a strong increase of more than 2-fold for the nanotip. Accompanying finite-difference time-domain (FDTD) simulations show a good match with the experimentally extracted near-field strengths. Additionally, high electric field localization for the nanotip is found. The combination of transmission electron microscope imaging of such nanotips and the determination of the near-field enhancement by electron rescattering represent a full characterization of the electric near-field of these intriguing electron emitters. Ultimately, nanotips as small as single nanometers can be produced, which is of utmost interest for electron diffraction experiments and low-emittance electron sources.
ISSN:1530-6984
1530-6992
DOI:10.1021/acs.nanolett.3c01985