High-flux wavelength tunable XUV source in the 12-40.8 eV photon energy range with adjustable energy and time resolution for Tr-ARPES applications

High-order harmonic generation (HHG) has a broad spectrum covering vacuum ultraviolet to extreme ultraviolet (XUV) bands, which is useful for applications involving material analyses at different information depths. Such an HHG light source is perfect for time- and angle-resolved photoemission spect...

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Veröffentlicht in:Optics express 2023-03, Vol.31 (6), p.9854-9871
Hauptverfasser: Wang, Ji, Chen, Famin, Pan, Mojun, Xu, Siyuan, Lv, Renchong, Liu, Junde, Li, Yuanfeng, Fang, Shaobo, Chen, Yunlin, Zhu, Jiangfeng, Zhang, Dacheng, Qian, Tian, Yun, Chenxia, Zhao, Kun, Ding, Hong, Wei, Zhiyi
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Sprache:eng
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Zusammenfassung:High-order harmonic generation (HHG) has a broad spectrum covering vacuum ultraviolet to extreme ultraviolet (XUV) bands, which is useful for applications involving material analyses at different information depths. Such an HHG light source is perfect for time- and angle-resolved photoemission spectroscopy. Here, we demonstrate a high-photon flux HHG source driven by a two-color field. Applying a fused silica compression stage to reduce the driving pulse width, we obtained a high XUV photon flux of 2 × 10 phs/s @21.6 eV on target. We designed a classical diffraction mounted (CDM) grating monochromator that can achieve a wide range of photon energy from 12 to 40.8 eV, while the time resolution is improved by reducing the pulse front tilt after the harmonic selection. We designed a spatial filtering method to adjust the time resolution using the CDM monochromator and significantly reduced the pulse front tilt of the XUV pulses. We also demonstrate a detailed prediction of the energy resolution broadening which is caused by the space charge effect.
ISSN:1094-4087
1094-4087
DOI:10.1364/OE.484088