Tunable cyano substituents in D–A conjugated polymers accessed via direct arylation for photocatalytic hydrogen production

Tunable cyano substituents in D–A conjugated polymers accessed via direct arylation for photocatalytic hydrogen production

2-Styrylthiophene-based donor–acceptor linear conjugated polymers with tunable cyano substituents are atom-economically obtained via direct C–H arylation for platinum-free photocatalytic hydrogen production, affording a HER of up to 9.79 mmol h −1 g −1 .

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Veröffentlicht in:Chemical communications (Cambridge, England) England), 2022-11, Vol.58 (91), p.12680-12683
Hauptverfasser: Ye, Dong-Nai, Zhang, Yu-Jie, Tan, Zhi-Rong, Xing, Yu-Qin, Chen, Zhengwang, Qiu, Jia-Bin, Liu, Shi-Yong
Format: Artikel
Sprache:eng
Schlagworte:
Hydrogen production
Polymers
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Zusammenfassung:2-Styrylthiophene-based donor–acceptor linear conjugated polymers with tunable cyano substituents are atom-economically obtained via direct C–H arylation for platinum-free photocatalytic hydrogen production, affording a HER of up to 9.79 mmol h −1 g −1 .
ISSN:1359-7345
1364-548X
DOI:10.1039/d2cc04625c