Research on the geochemical background values and evolution rules of lake sediments for heavy metals and nutrients in the Eastern China Plain from 1937 to 2017

For the first time, background quality guidelines have been developed for lake sediments along the Yangtze River. Evolution Rules of watershed environment in Eastern China were analyzed in 1937–2017. These methods of 137Cs and 210Pb radionuclide, 75% cumulative frequency, and background method were...

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Veröffentlicht in:Journal of hazardous materials 2022-08, Vol.436, p.129136-129136, Article 129136
Hauptverfasser: Luo, Mingke, Kang, Xiaoqi, Liu, Qian, Yu, Hui, Tao, Yanru, Wang, Haonan, Niu, Yong, Niu, Yuan
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Sprache:eng
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Zusammenfassung:For the first time, background quality guidelines have been developed for lake sediments along the Yangtze River. Evolution Rules of watershed environment in Eastern China were analyzed in 1937–2017. These methods of 137Cs and 210Pb radionuclide, 75% cumulative frequency, and background method were applied to calculate the sediment geochemical backgrounds (GB). The average GB values of Cu, Zn, Cd, Pb, Cr, total carbon (TC), total nitrogen (TN) and total phosphorus (TP) are 45.14 mg/kg, 86.99 mg/kg, 0.29 mg/kg, 33.71 mg/kg, 110.90 mg/kg, 17.20 mg/g, 1.60 mg/g, and 665.78 mg/kg, respectively. The radionuclide methods indicated that the sediment rate of 34 cm corresponding to 1963 is 0.63 cm yr−1. The risk and accumulation of the sediment metals and nutrients in Yangtze Plain were uncontaminated levels before 1960, raised since 1980, and increased significantly in 2000. The Cd, TC, and TN in lake sediment were at low to moderate pollution, and few lakes are at high pollution. Sediment background values of the plain are different from soil background values in China and Consensus-Based Sediment Quality Guidelines in Europe/America. Results of sediment quality guidelines provide an important guidance for pollution prevention, environmental management, and risk assessment, especially the formulation of environmental laws. [Display omitted] •1.137Cs and 210Pb method were used to study the Sediment geochemical backgrounds.•2. Cd was the main pollutant in whole Yangtze basin.•3. Sediment depth of 4.4, 23.3, and 42 cm corresponded 2010, 1980, and 1950 year.•4. Risk evaluation and environmental management by soil values are not accurate.
ISSN:0304-3894
1873-3336
DOI:10.1016/j.jhazmat.2022.129136