Ultra-stretchable, super-hydrophobic and high-conductive composite for wearable strain sensors with high sensitivity

[Display omitted] With continuous development of artificial intelligence technology, strain sensors have attracted widespread attention. In this work, a novel high-performance wearable strain sensor is prepared by using a kind of ultra-stretchable, super-hydrophobic and high-conductive composite. The preparation process is as follows, i.e., using common elastic band (EB) as the polymer matrix, nano carbon black (CB) and carbon nanotubes (CNTs) as mixed conductive filler, and then modified by polydimethylsiloxane (PDMS) to obtain the PDMS/(CB + CNTs)/EB composite for assembling assemble flexible wearable strain sensors. Experimental results reveal the following excellent properties: 1) The composite exhibits excellent mechanical properties and super-hydrophobicity, i.e., the tensile strength is up to 996.5%, and the elastic modulus and tensile strength increase 49.2% and 59.2%, compared with pristine EB; 2) The composite strain sensor exhibits high sensitivity (the gauge factor reaches up to 648.83 under strain range of 979.9–996.5%), and it still shows stable performance after 3000 cycles tests (100% strain); 3) It is a well candidate to be used for monitoring human body motions including large and subtle body movements; 4) The composite sensor also has advantages of easy access of raw materials, simple preparation, easy mass production and relatively low production cost, showing a broad application prospect in wearable electronic products.