Barrier Crossing in a Viscoelastic Bath

We investigate the hopping dynamics of a colloidal particle across a potential barrier and within a viscoelastic, i.e., non-Markovian, bath and report two clearly separated timescales in the corresponding waiting time distributions. While the longer timescale exponentially depends on the barrier hei...

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Veröffentlicht in:Physical review letters 2022-01, Vol.128 (2), p.028001-028001, Article 028001
Hauptverfasser: Ginot, Félix, Caspers, Juliana, Krüger, Matthias, Bechinger, Clemens
Format: Artikel
Sprache:eng
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Zusammenfassung:We investigate the hopping dynamics of a colloidal particle across a potential barrier and within a viscoelastic, i.e., non-Markovian, bath and report two clearly separated timescales in the corresponding waiting time distributions. While the longer timescale exponentially depends on the barrier height, the shorter one is similar to the relaxation time of the fluid. This short timescale is a signature of the storage and release of elastic energy inside the bath that strongly increases the hopping rate. Our results are in excellent agreement with numerical simulations of a simple Maxwell model.
ISSN:0031-9007
1079-7114
DOI:10.1103/PhysRevLett.128.028001