Barrier Crossing in a Viscoelastic Bath
We investigate the hopping dynamics of a colloidal particle across a potential barrier and within a viscoelastic, i.e., non-Markovian, bath and report two clearly separated timescales in the corresponding waiting time distributions. While the longer timescale exponentially depends on the barrier hei...
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Veröffentlicht in: | Physical review letters 2022-01, Vol.128 (2), p.028001-028001, Article 028001 |
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Hauptverfasser: | , , , |
Format: | Artikel |
Sprache: | eng |
Online-Zugang: | Volltext |
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Zusammenfassung: | We investigate the hopping dynamics of a colloidal particle across a potential barrier and within a viscoelastic, i.e., non-Markovian, bath and report two clearly separated timescales in the corresponding waiting time distributions. While the longer timescale exponentially depends on the barrier height, the shorter one is similar to the relaxation time of the fluid. This short timescale is a signature of the storage and release of elastic energy inside the bath that strongly increases the hopping rate. Our results are in excellent agreement with numerical simulations of a simple Maxwell model. |
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ISSN: | 0031-9007 1079-7114 |
DOI: | 10.1103/PhysRevLett.128.028001 |