Emerging Long‐Range Order from a Freeform Disordered Metasurface

Recently, disordered metasurfaces have attracted considerable interest due to their potential applications in imaging, holography, and wavefront shaping. However, how to emerge long‐range ordered phase distribution in disordered metasurfaces remains an outstanding problem. Here, a general framework is proposed to generate a spatially homogeneous in‐plane phase distribution from a disordered metasurface, by engineering disorder parameters together with topology optimization. As a proof‐of‐concept demonstration, an all‐dielectric disordered supercell metasurface with relatively homogeneous in‐plane phase fluctuation is designed by disorder parameter engineering, manifesting as polarization conversion‐dependent random scattering or unidirectional transmission. Then, a topology optimization approach is utilized to overcome the lattice coupling effect and to further improve the homogeneity of complex electric field fluctuation. In comparison with the initial supercell metasurface, both the phase fluctuation range and the relative efficiency of the topology‐optimized freeform metasurface are significantly improved, leading to a long‐range ordered electric field distribution. Moreover, three experimental realizations are performed, all of which agree well with the theoretical results. This methodology may inspire more exotic optical phenomena and find more promising applications in disordered metasurfaces and disordered optics. A general framework for emerging long‐range ordered phase distribution in a freeform disordered metasurface is established based on disorder parameter engineering and topology optimization. Within this general framework, the order distribution and the corresponding functionality can be inversely optimized and artificially designed, offering a new freedom to design material functionality.