Dual Active Centers Bridged by Oxygen Vacancies of Ruthenium Single‐Atom Hybrids Supported on Molybdenum Oxide for Photocatalytic Ammonia Synthesis

Dual Active Centers Bridged by Oxygen Vacancies of Ruthenium Single‐Atom Hybrids Supported on Molybdenum Oxide for Photocatalytic Ammonia Synthesis

Photocatalytic synthesis of ammonia (NH3) holds significant potential compared with the Haber–Bosch process. However, the reported photocatalysts suffer from low efficiency owing to localized electron deficiency. Herein, Ru‐SA (single atoms)/HxMoO3−y hybrids with abundant of Mon+ (4

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Veröffentlicht in:Angewandte Chemie International Edition 2022-03, Vol.61 (14), p.e202114242-n/a
Hauptverfasser: Yin, Haibo, Chen, Zhen, Peng, Yue, Xiong, Shangchao, Li, Yadong, Yamashita, Hiromi, Li, Junhua
Format: Artikel
Sprache:eng
Schlagworte:
Ammonia
Dual active centers
H-spillover
Haber Bosch process
Hybrids
Molybdenum
Molybdenum oxides
NH3 synthesis
Oxygen
Photocatalysis
Photocatalytic
Quantum efficiency
Ru single atom hybrids
Ruthenium
Synthesis
Vacancies
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Zusammenfassung:Photocatalytic synthesis of ammonia (NH3) holds significant potential compared with the Haber–Bosch process. However, the reported photocatalysts suffer from low efficiency owing to localized electron deficiency. Herein, Ru‐SA (single atoms)/HxMoO3−y hybrids with abundant of Mon+ (4
ISSN:1433-7851
1521-3773
DOI:10.1002/anie.202114242