Research progress of smart response composite hydrogels based on nanocellulose

In recent years, smart-responsive nanocellulose composite hydrogels have attracted extensive attention due to their unique porous substrate, hydrophilic properties, biocompatibility and stimulus responsiveness. At present, the research on smart response nanocellulose composite hydrogel mainly focuses on the selection of composite materials and the construction of internal chemical bonds. The common composite materials and connection methods used for preparation of smart response nanocellulose composite hydrogels are compared according to the different types of response sources such as temperature, pH and so on. The response mechanisms and the application prospects of different response types of nanocellulose composite hydrogels are summarized, and the transformation of internal ions, functional groups and chemical bonds, as well as the changes in mechanical properties such as modulus and strength are discussed. Finally, the shortcomings and application prospects of nanocellulose smart response composite hydrogels are summarized and prospected. •Nanocellulose has the advantages of mechanical properties.•Nanocellulose composite hydrogels have a variety of response characteristics through composite different materials.•The characteristic of nanocellulose composite hydrogels is analyzed according to the mechanism.•Nanocellulose can significantly improve the strength and modulus of hydrogels.