Modulation of Spin–Orbit Torque from SrRuO3 by Epitaxial‐Strain‐Induced Octahedral Rotation

Spin–orbit torque (SOT), which arises from the spin–orbit coupling of conduction electrons, is believed to be the key route for developing low‐power, high‐speed, and nonvolatile memory devices. Despite the theoretical prediction of pronounced Berry phase curvatures in certain transition‐metal perovskite oxides, which lead to considerable intrinsic spin Hall conductivity, SOT from this class of materials has rarely been reported until recently. Here, the SOT generated by epitaxial SrRuO3 of three different crystal structures is systematically studied. The results of both spin‐torque ferromagnetic resonance and in‐plane harmonic Hall voltage measurements concurrently reveal that the intrinsic SOT efficiency of SrRuO3 decreases when the epitaxial strain changes from tensile to compressive. The X‐ray diffraction data demonstrate a strong correlation between the magnitude of SOT and octahedral rotation around the in‐plane axes of SrRuO3, consistent with the theoretical prediction. This work offers new possibilities of tuning SOT with crystal structures and novel opportunities of integrating the unique properties of perovskite oxides with spintronic functionalities. Transition metal oxide perovskite oxides can have pronounced Berry phase curvatures and moderate electric conductivity, making them good sources of spin–orbit torque. The spin–orbit torque efficiency of SrRuO3 of three different crystal phases is investigated. Both experimental and theoretical results suggest that the spin–orbit torque efficiency is strongly correlated to the in‐plane octahedral rotation in SrRuO3.