The level, distribution and source of artificial radionuclides in surface soil from Inner Mongolia, China

Mid- and long-half-life artificial radioisotopes in the earth's surface environment are of great concern to the environmental radiation risk assessment. As nuclear fuel and fission products, 239Pu, 240Pu, 241Am, 90Sr and 137Cs in soils from Inner Mongolia of China were analyzed with a modified systematic separation procedure combined with ICP-MS and LSC measurements, to study the level, distribution and source of artificial radionuclides in the region. The radioactivity and inventory of 137Cs (0.26–28.3 Bq/kg, 0.5–5.4 kBq/m2), 239+240Pu (0.05–1.26 Bq/kg, 20-229 Bq/m2), 241Am (0.036–0.35 Bq/kg, 11-81 Bq/m2) and 90Sr (1.2–7.6 Bq/kg, 0.39–1.7 kBq/m2) all lie in the range of the global fallout. Vertical distributions of these radionuclides were examined for two soil core samples SC14025 and SC14038, and great differences were observed between these two sample locations. For SC14025 where little human disturbance to soil occurred, both 137Cs and 239+240Pu have a subsurface activity maximum followed by an exponential decay. Fittings base on CDE model gives a small downward migration velocity of about 0.097 cm/y for both Pu and 137Cs. Source identification for SC14025 and SC14038 soil cores with 240Pu/239Pu (average of 0.180 ± 0.017 and 0.164 ± 0.035, respectively), 137Cs/239+240Pu (average of 25.3 ± 0.6 and 25.6 ± 3.0, respectively) and 241Am/239+240Pu (average of 0.56 ± 0.08 and 0.60 ± 0.09, respectively) ratios consistently indicated that anthropogenic radionuclides in Xilingol region are mostly from the global fallout of atmospheric nuclear weapons tests in the last century. According to the geographical distribution of the radioactivity level, the high radioactivity level in the east of Inner Mongolia probably results from enhanced deposition by the blocking of the Great Khingan Range. •Multi-fingerprints indicate the radionuclides in studied areas are mostly from the global fallout.•Downward migration of 239Pu and 137Cs is similar and low while 90Sr migrates much faster.•High radioactivity level might result from enhanced deposition by mountain blocking.