High-Performance, Thermal Cycling Stable, Coking-Tolerant Solid Oxide Fuel Cells with Nanostructured Electrodes
Solid oxide fuel cells (SOFCs) are a promising solution to a sustainable energy future. However, cell performance and stability remain a challenge. Durable, nanostructured electrodes fabricated via a simple, cost-effective method are an effective way to address these problems. In this work, both the...
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| Veröffentlicht in: | ACS applied materials & interfaces 2021-02, Vol.13 (4), p.4993-4999 |
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| creator | Zhang, Weilin Zhou, Yucun Hussain, A. Mohammed Song, Dong Miura, Yohei Chen, Yu Luo, Zheyu Kane, Nicholas Niu, Yinghua Dale, Nilesh Fukuyama, Yosuke Liu, Meilin |
| description | Solid oxide fuel cells (SOFCs) are a promising solution to a sustainable energy future. However, cell performance and stability remain a challenge. Durable, nanostructured electrodes fabricated via a simple, cost-effective method are an effective way to address these problems. In this work, both the nanostructured PrBa0.5Sr0.5Co1.5Fe0.5O5+δ (PBSCF) cathode and Ni–Ce0.8Sm0.2O1.9 (SDC) anode are fabricated on a porous yttria-stabilized zirconia (YSZ) backbone via solution infiltration. Symmetrical cells with a configuration of PBSCF|YSZ|PBSCF show a low interfacial polarization resistance of 0.03 Ω cm2 with minimal degradation at 700 °C for 600 h. Ni-SDC|YSZ|PBSCF single cells exhibit a peak power density of 0.62 W cm–2 at 650 °C operated on H2 with good thermal cycling stability for 110 h. Single cells also show excellent coking tolerance with stable operation on CH4 for over 120 h. This work offers a promising pathway toward the development of high-performance and durable SOFCs to be powered by natural gas. |
| doi_str_mv | 10.1021/acsami.0c18434 |
| format | Article |
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Mohammed ; Song, Dong ; Miura, Yohei ; Chen, Yu ; Luo, Zheyu ; Kane, Nicholas ; Niu, Yinghua ; Dale, Nilesh ; Fukuyama, Yosuke ; Liu, Meilin</creator><creatorcontrib>Zhang, Weilin ; Zhou, Yucun ; Hussain, A. Mohammed ; Song, Dong ; Miura, Yohei ; Chen, Yu ; Luo, Zheyu ; Kane, Nicholas ; Niu, Yinghua ; Dale, Nilesh ; Fukuyama, Yosuke ; Liu, Meilin</creatorcontrib><description>Solid oxide fuel cells (SOFCs) are a promising solution to a sustainable energy future. However, cell performance and stability remain a challenge. Durable, nanostructured electrodes fabricated via a simple, cost-effective method are an effective way to address these problems. In this work, both the nanostructured PrBa0.5Sr0.5Co1.5Fe0.5O5+δ (PBSCF) cathode and Ni–Ce0.8Sm0.2O1.9 (SDC) anode are fabricated on a porous yttria-stabilized zirconia (YSZ) backbone via solution infiltration. Symmetrical cells with a configuration of PBSCF|YSZ|PBSCF show a low interfacial polarization resistance of 0.03 Ω cm2 with minimal degradation at 700 °C for 600 h. Ni-SDC|YSZ|PBSCF single cells exhibit a peak power density of 0.62 W cm–2 at 650 °C operated on H2 with good thermal cycling stability for 110 h. Single cells also show excellent coking tolerance with stable operation on CH4 for over 120 h. 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Mohammed</creatorcontrib><creatorcontrib>Song, Dong</creatorcontrib><creatorcontrib>Miura, Yohei</creatorcontrib><creatorcontrib>Chen, Yu</creatorcontrib><creatorcontrib>Luo, Zheyu</creatorcontrib><creatorcontrib>Kane, Nicholas</creatorcontrib><creatorcontrib>Niu, Yinghua</creatorcontrib><creatorcontrib>Dale, Nilesh</creatorcontrib><creatorcontrib>Fukuyama, Yosuke</creatorcontrib><creatorcontrib>Liu, Meilin</creatorcontrib><title>High-Performance, Thermal Cycling Stable, Coking-Tolerant Solid Oxide Fuel Cells with Nanostructured Electrodes</title><title>ACS applied materials & interfaces</title><addtitle>ACS Appl. Mater. Interfaces</addtitle><description>Solid oxide fuel cells (SOFCs) are a promising solution to a sustainable energy future. However, cell performance and stability remain a challenge. Durable, nanostructured electrodes fabricated via a simple, cost-effective method are an effective way to address these problems. 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| title | High-Performance, Thermal Cycling Stable, Coking-Tolerant Solid Oxide Fuel Cells with Nanostructured Electrodes |
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