Adhesion Enhancement of Micropillar Array by Combining the Adhesive Design from Gecko and Tree Frog

It has long been demonstrated the gecko‐inspired micropillar array with T‐shape tips possesses the best adhesion performance of a given material. The further enhancement of the adhesion performances of T‐shape micropillars can offer redundant adhesion to compensate for the inevitable improper contacts. Here, the array of T‐shape polydimethylsiloxane (PDMS) micropillars is incorporated with gradient dispersed calcium carbonate nanoparticles in the micropillar stalk, termed as T‐shape gradient micropillars (TG), possessing the modulus gradient with stiff tip and soft root. The gradient modulus in TG facilitates the contact formation and regulates the stress at the detaching interface, resulting in a 4.6 times adhesion and 2.4 times friction as compared with the pure PDMS T‐shape micropillar arrays. The study here provides a new design strategy for the super‐strong structured dry adhesives. An array of T‐shape gradient micropillars is developed by combining the T‐shape tips inspired by gecko setae and the modulus gradient found in tree frogs. The gradient modulus facilitates the contact formation and regulates the stress distribution at the detaching interface, resulting in a 4.6 times adhesion and a 2.4 times friction as compared with the T‐shape polydimethylsiloxane micropillar array.