Coherent Control of Internal Conversion in Strong-Field Molecular Ionization
We demonstrate coherent control over internal conversion during strong-field molecular ionization with shaped, few-cycle laser pulses. The control is driven by interference in different neutral states, which are coupled via non-Born-Oppenheimer terms in the molecular Hamiltonian. Our measurements hi...
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Veröffentlicht in: | Physical review letters 2020-07, Vol.125 (5), p.1-053202, Article 053202 |
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Format: | Artikel |
Sprache: | eng |
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Zusammenfassung: | We demonstrate coherent control over internal conversion during strong-field molecular ionization with shaped, few-cycle laser pulses. The control is driven by interference in different neutral states, which are coupled via non-Born-Oppenheimer terms in the molecular Hamiltonian. Our measurements highlight the preservation of electronic coherence in nonadiabatic transitions between electronic states. |
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ISSN: | 0031-9007 1079-7114 |
DOI: | 10.1103/PhysRevLett.125.053202 |