Size distribution of particulate matter in runoff from different leaf surfaces during controlled rainfall processes

The presence of plant leaves has been shown to lower the risks of health problems by reducing atmospheric particulate matter (PM). Leaf PM accumulation capacity will saturate in the absence of runoff. Rainfall is an effective way for PM to “wash off” into the soil and renew leaf PM accumulation. However, little is known about how PM wash-off varies with PM size and health problems caused by particulate pollution vary with PM size. This study thus used artificial rainfall with six plant species to find out how size-fractioned PM are washed off during rain processes. Total wash-off masses in fine, coarse and large fractions were 0.6–10.3 μg/cm2, 1.0–18.8 μg/cm2 and 4.5–60.1 μg/cm2 respectively. P. orientalis (cypress) and E. japonicus (evergreen broadleaved shrub) had the largest wash-off masses in each fraction during rainfall. P. cerasifera (deciduous broadleaved shrub) had the largest cumulative wash-off rates in each fraction. Rainfall intensity had more influence on wash-off masses and rates of large particles for six species and for small particles in evergreen species, but limited effect on wash-off proportions. Wash-off proportions decreased in large particles and increased in small particles along with rainfall. The results provide information for PM accumulation renewal of plants used for urban greening. [Display omitted] •Wash-off masses of large particles increased by rainfall intensity.•Wash-off rates of small particles increased by intensity for evergreen plants.•Large fractions were washed off preferentially in early rainfall.•Wash-off dynamics of three size fractions differed among plant species. Size distribution of PM wash-off dynamics during rainfall processes differed among plant species, rainfall intensities and intervals.