Construction of Spatial Charge Separation Facets on BaTaO2N Crystals by Flux Growth Approach for Visible-Light-Driven H2 Production
Low charge separation efficiencies are regarded as obstacles that limit the improvement in the photocatalytic performance of BaTaO2N. In this study, we demonstrated that the anisotropic facets ({100} and {110} facets) of BaTaO2N for efficient spatial charge separation were successfully constructed u...
Gespeichert in:
Veröffentlicht in: | ACS applied materials & interfaces 2019-06, Vol.11 (25), p.22264-22271 |
---|---|
Hauptverfasser: | , , , , , , , , , |
Format: | Artikel |
Sprache: | eng |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | 22271 |
---|---|
container_issue | 25 |
container_start_page | 22264 |
container_title | ACS applied materials & interfaces |
container_volume | 11 |
creator | Luo, Ying Suzuki, Sayaka Wang, Zheng Yubuta, Kunio Vequizo, Junie Jhon M Yamakata, Akira Shiiba, Hiromasa Hisatomi, Takashi Domen, Kazunari Teshima, Katsuya |
description | Low charge separation efficiencies are regarded as obstacles that limit the improvement in the photocatalytic performance of BaTaO2N. In this study, we demonstrated that the anisotropic facets ({100} and {110} facets) of BaTaO2N for efficient spatial charge separation were successfully constructed using the one-pot flux-assisted nitridation approach. As a result, the photocatalytic activity for H2 production on BaTaO2N with coexposed {100} and {110} facets was nearly 10-fold over that of BaTaO2N with only {100} facets and that of the conventional irregularly shaped sample. This finding provides an innovative approach to the development of efficient (oxy)nitride photocatalysts for solar energy conversion. |
doi_str_mv | 10.1021/acsami.9b03747 |
format | Article |
fullrecord | <record><control><sourceid>proquest_acs_j</sourceid><recordid>TN_cdi_proquest_miscellaneous_2233856165</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2233856165</sourcerecordid><originalsourceid>FETCH-LOGICAL-a204t-771e7d82834e75879f890430a5c95f6b45ab8cb8ffc068a88af186b6ee2782d43</originalsourceid><addsrcrecordid>eNo9kMFLwzAYxYsoOKdXzzmK0JmkaZMeZ3WbMJyw6bV8zZK1o2tmkqo7-49b7fD0Pfge7z1-QXBN8IhgSu5AOthVo7TAEWf8JBiQlLFQ0Jie_mvGzoML57YYJxHF8SD4zkzjvG2lr0yDjEbLPfgKapSVYDcKLdUeLPw9JyCVd6hT97CCBX1GmT04D7VDxQFN6vYLTa359CUa7_fWgCyRNha9Va4qahXOq03pwwdbfagGzSh6sWbd114GZ7pLUVfHOwxeJ4-rbBbOF9OnbDwPgWLmQ86J4mtBRcQUjwVPtUgxizDEMo11UrAYCiELobXEiQAhQBORFIlSlAu6ZtEwuOlzu3XvrXI-31VOqrqGRpnW5ZRGkYgTksSd9ba3dlDzrWlt0w3LCc5_Sec96fxIOvoBaaJzEg</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2233856165</pqid></control><display><type>article</type><title>Construction of Spatial Charge Separation Facets on BaTaO2N Crystals by Flux Growth Approach for Visible-Light-Driven H2 Production</title><source>ACS Publications</source><creator>Luo, Ying ; Suzuki, Sayaka ; Wang, Zheng ; Yubuta, Kunio ; Vequizo, Junie Jhon M ; Yamakata, Akira ; Shiiba, Hiromasa ; Hisatomi, Takashi ; Domen, Kazunari ; Teshima, Katsuya</creator><creatorcontrib>Luo, Ying ; Suzuki, Sayaka ; Wang, Zheng ; Yubuta, Kunio ; Vequizo, Junie Jhon M ; Yamakata, Akira ; Shiiba, Hiromasa ; Hisatomi, Takashi ; Domen, Kazunari ; Teshima, Katsuya</creatorcontrib><description>Low charge separation efficiencies are regarded as obstacles that limit the improvement in the photocatalytic performance of BaTaO2N. In this study, we demonstrated that the anisotropic facets ({100} and {110} facets) of BaTaO2N for efficient spatial charge separation were successfully constructed using the one-pot flux-assisted nitridation approach. As a result, the photocatalytic activity for H2 production on BaTaO2N with coexposed {100} and {110} facets was nearly 10-fold over that of BaTaO2N with only {100} facets and that of the conventional irregularly shaped sample. This finding provides an innovative approach to the development of efficient (oxy)nitride photocatalysts for solar energy conversion.</description><identifier>ISSN: 1944-8244</identifier><identifier>EISSN: 1944-8252</identifier><identifier>DOI: 10.1021/acsami.9b03747</identifier><language>eng</language><publisher>American Chemical Society</publisher><ispartof>ACS applied materials & interfaces, 2019-06, Vol.11 (25), p.22264-22271</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><orcidid>0000-0003-3179-7588 ; 0000-0001-7995-4832 ; 0000-0002-0186-1959 ; 0000-0002-5009-2383 ; 0000-0002-5784-5157</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acsami.9b03747$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acsami.9b03747$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,776,780,27053,27901,27902,56713,56763</link.rule.ids></links><search><creatorcontrib>Luo, Ying</creatorcontrib><creatorcontrib>Suzuki, Sayaka</creatorcontrib><creatorcontrib>Wang, Zheng</creatorcontrib><creatorcontrib>Yubuta, Kunio</creatorcontrib><creatorcontrib>Vequizo, Junie Jhon M</creatorcontrib><creatorcontrib>Yamakata, Akira</creatorcontrib><creatorcontrib>Shiiba, Hiromasa</creatorcontrib><creatorcontrib>Hisatomi, Takashi</creatorcontrib><creatorcontrib>Domen, Kazunari</creatorcontrib><creatorcontrib>Teshima, Katsuya</creatorcontrib><title>Construction of Spatial Charge Separation Facets on BaTaO2N Crystals by Flux Growth Approach for Visible-Light-Driven H2 Production</title><title>ACS applied materials & interfaces</title><addtitle>ACS Appl. Mater. Interfaces</addtitle><description>Low charge separation efficiencies are regarded as obstacles that limit the improvement in the photocatalytic performance of BaTaO2N. In this study, we demonstrated that the anisotropic facets ({100} and {110} facets) of BaTaO2N for efficient spatial charge separation were successfully constructed using the one-pot flux-assisted nitridation approach. As a result, the photocatalytic activity for H2 production on BaTaO2N with coexposed {100} and {110} facets was nearly 10-fold over that of BaTaO2N with only {100} facets and that of the conventional irregularly shaped sample. This finding provides an innovative approach to the development of efficient (oxy)nitride photocatalysts for solar energy conversion.</description><issn>1944-8244</issn><issn>1944-8252</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNo9kMFLwzAYxYsoOKdXzzmK0JmkaZMeZ3WbMJyw6bV8zZK1o2tmkqo7-49b7fD0Pfge7z1-QXBN8IhgSu5AOthVo7TAEWf8JBiQlLFQ0Jie_mvGzoML57YYJxHF8SD4zkzjvG2lr0yDjEbLPfgKapSVYDcKLdUeLPw9JyCVd6hT97CCBX1GmT04D7VDxQFN6vYLTa359CUa7_fWgCyRNha9Va4qahXOq03pwwdbfagGzSh6sWbd114GZ7pLUVfHOwxeJ4-rbBbOF9OnbDwPgWLmQ86J4mtBRcQUjwVPtUgxizDEMo11UrAYCiELobXEiQAhQBORFIlSlAu6ZtEwuOlzu3XvrXI-31VOqrqGRpnW5ZRGkYgTksSd9ba3dlDzrWlt0w3LCc5_Sec96fxIOvoBaaJzEg</recordid><startdate>20190626</startdate><enddate>20190626</enddate><creator>Luo, Ying</creator><creator>Suzuki, Sayaka</creator><creator>Wang, Zheng</creator><creator>Yubuta, Kunio</creator><creator>Vequizo, Junie Jhon M</creator><creator>Yamakata, Akira</creator><creator>Shiiba, Hiromasa</creator><creator>Hisatomi, Takashi</creator><creator>Domen, Kazunari</creator><creator>Teshima, Katsuya</creator><general>American Chemical Society</general><scope>7X8</scope><orcidid>https://orcid.org/0000-0003-3179-7588</orcidid><orcidid>https://orcid.org/0000-0001-7995-4832</orcidid><orcidid>https://orcid.org/0000-0002-0186-1959</orcidid><orcidid>https://orcid.org/0000-0002-5009-2383</orcidid><orcidid>https://orcid.org/0000-0002-5784-5157</orcidid></search><sort><creationdate>20190626</creationdate><title>Construction of Spatial Charge Separation Facets on BaTaO2N Crystals by Flux Growth Approach for Visible-Light-Driven H2 Production</title><author>Luo, Ying ; Suzuki, Sayaka ; Wang, Zheng ; Yubuta, Kunio ; Vequizo, Junie Jhon M ; Yamakata, Akira ; Shiiba, Hiromasa ; Hisatomi, Takashi ; Domen, Kazunari ; Teshima, Katsuya</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a204t-771e7d82834e75879f890430a5c95f6b45ab8cb8ffc068a88af186b6ee2782d43</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Luo, Ying</creatorcontrib><creatorcontrib>Suzuki, Sayaka</creatorcontrib><creatorcontrib>Wang, Zheng</creatorcontrib><creatorcontrib>Yubuta, Kunio</creatorcontrib><creatorcontrib>Vequizo, Junie Jhon M</creatorcontrib><creatorcontrib>Yamakata, Akira</creatorcontrib><creatorcontrib>Shiiba, Hiromasa</creatorcontrib><creatorcontrib>Hisatomi, Takashi</creatorcontrib><creatorcontrib>Domen, Kazunari</creatorcontrib><creatorcontrib>Teshima, Katsuya</creatorcontrib><collection>MEDLINE - Academic</collection><jtitle>ACS applied materials & interfaces</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Luo, Ying</au><au>Suzuki, Sayaka</au><au>Wang, Zheng</au><au>Yubuta, Kunio</au><au>Vequizo, Junie Jhon M</au><au>Yamakata, Akira</au><au>Shiiba, Hiromasa</au><au>Hisatomi, Takashi</au><au>Domen, Kazunari</au><au>Teshima, Katsuya</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Construction of Spatial Charge Separation Facets on BaTaO2N Crystals by Flux Growth Approach for Visible-Light-Driven H2 Production</atitle><jtitle>ACS applied materials & interfaces</jtitle><addtitle>ACS Appl. Mater. Interfaces</addtitle><date>2019-06-26</date><risdate>2019</risdate><volume>11</volume><issue>25</issue><spage>22264</spage><epage>22271</epage><pages>22264-22271</pages><issn>1944-8244</issn><eissn>1944-8252</eissn><abstract>Low charge separation efficiencies are regarded as obstacles that limit the improvement in the photocatalytic performance of BaTaO2N. In this study, we demonstrated that the anisotropic facets ({100} and {110} facets) of BaTaO2N for efficient spatial charge separation were successfully constructed using the one-pot flux-assisted nitridation approach. As a result, the photocatalytic activity for H2 production on BaTaO2N with coexposed {100} and {110} facets was nearly 10-fold over that of BaTaO2N with only {100} facets and that of the conventional irregularly shaped sample. This finding provides an innovative approach to the development of efficient (oxy)nitride photocatalysts for solar energy conversion.</abstract><pub>American Chemical Society</pub><doi>10.1021/acsami.9b03747</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0003-3179-7588</orcidid><orcidid>https://orcid.org/0000-0001-7995-4832</orcidid><orcidid>https://orcid.org/0000-0002-0186-1959</orcidid><orcidid>https://orcid.org/0000-0002-5009-2383</orcidid><orcidid>https://orcid.org/0000-0002-5784-5157</orcidid></addata></record> |
fulltext | fulltext |
identifier | ISSN: 1944-8244 |
ispartof | ACS applied materials & interfaces, 2019-06, Vol.11 (25), p.22264-22271 |
issn | 1944-8244 1944-8252 |
language | eng |
recordid | cdi_proquest_miscellaneous_2233856165 |
source | ACS Publications |
title | Construction of Spatial Charge Separation Facets on BaTaO2N Crystals by Flux Growth Approach for Visible-Light-Driven H2 Production |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-02T07%3A35%3A50IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_acs_j&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Construction%20of%20Spatial%20Charge%20Separation%20Facets%20on%20BaTaO2N%20Crystals%20by%20Flux%20Growth%20Approach%20for%20Visible-Light-Driven%20H2%20Production&rft.jtitle=ACS%20applied%20materials%20&%20interfaces&rft.au=Luo,%20Ying&rft.date=2019-06-26&rft.volume=11&rft.issue=25&rft.spage=22264&rft.epage=22271&rft.pages=22264-22271&rft.issn=1944-8244&rft.eissn=1944-8252&rft_id=info:doi/10.1021/acsami.9b03747&rft_dat=%3Cproquest_acs_j%3E2233856165%3C/proquest_acs_j%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2233856165&rft_id=info:pmid/&rfr_iscdi=true |