Plasma catalytic oxidation of toluene over double perovskite-type oxide via packed-bed DBD
Various perovskite-type catalysts including La 2 CoMnO 6 , LaCoO 3 , and LaMnO 3 are first evaluated for the activities toward C 7 H 8 removal. Experimental results indicate that double-type La 2 CoMnO 6 shows better activity if compared with single perovskites due to high lattice oxygen content and...
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| creator | Pan, Kuan Lun Chang, Moo Been |
| description | Various perovskite-type catalysts including La
2
CoMnO
6
, LaCoO
3
, and LaMnO
3
are first evaluated for the activities toward C
7
H
8
removal. Experimental results indicate that double-type La
2
CoMnO
6
shows better activity if compared with single perovskites due to high lattice oxygen content and good reducibility. Subsequently, perovskite catalysts are combined with plasma (NTP) to form in-plasma catalysis (IPC) and post-plasma catalysis (PPC) systems. The results indicate that IPC systems have better higher performance than that of NTP-alone and PPC. Especially, high C
7
H
8
conversion (100%) and mineralization efficiency (96.8%) can be achieved with the applied voltage of 18 kV and temperature of 120 °C when La
2
CoMnO
6
is integrated with NTP to form IPC system. Also, it owns the highest energy efficiency (0.14 g/kWh). It is concluded that IPC performance for C
7
H
8
removal is closely related with the properties of catalyst surface. In addition, the kinetics of IPC systems are investigated by a simplified model, and the result indicates that IPC with La
2
CoMnO
6
as catalyst has a higher overall energy constant. This study reveals that double-type La
2
CoMnO
6
is of higher activity than single perovskites for C
7
H
8
removal, and demonstrates that double-type La
2
CoMnO
6
is of high potential to form plasma catalysis system for VOCs removal. |
| doi_str_mv | 10.1007/s11356-019-04714-0 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_2195262249</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2194435222</sourcerecordid><originalsourceid>FETCH-LOGICAL-c412t-7b548e80dd6fd7f2a57912988a4ebf5808e28937c7d78b5b696f3900d625fd7d3</originalsourceid><addsrcrecordid>eNp9kE1v1DAQhi1ERbeFP8ABWeLCxe3YsWP72O8iVYIDXLhYTjxBabNxaicr9t_X7RYqcejJI_l53xk9hHzkcMQB9HHmvFI1A24ZSM0lgzdkxesyaGntW7ICKyXjlZT75CDnWwABVuh3ZL8CY5WSekV-fR98Xnva-tkP27lvafzTBz_3caSxo3McFhyRxg0mGuLSDEgnTHGT7_oZ2byd8CmAdNN7Ovn2DgNrMNDz0_P3ZK_zQ8YPz-8h-Xl58ePsmt18u_p6dnLDWsnFzHSjpEEDIdRd0J3wSlsurDFeYtMpAwaFsZVuddCmUU1t666yAKEWqgRCdUi-7HqnFO8XzLNb97nFYfAjxiU7wa0StRDSFvTzf-htXNJYrnukpKyUEKJQYke1KeacsHNT6tc-bR0H92je7cy7Yt49mXdQQp-eq5dmjeFf5K_qAlQ7IJev8Teml92v1D4APveNgQ</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2194435222</pqid></control><display><type>article</type><title>Plasma catalytic oxidation of toluene over double perovskite-type oxide via packed-bed DBD</title><source>MEDLINE</source><source>SpringerLink Journals - AutoHoldings</source><creator>Pan, Kuan Lun ; Chang, Moo Been</creator><creatorcontrib>Pan, Kuan Lun ; Chang, Moo Been</creatorcontrib><description>Various perovskite-type catalysts including La
2
CoMnO
6
, LaCoO
3
, and LaMnO
3
are first evaluated for the activities toward C
7
H
8
removal. Experimental results indicate that double-type La
2
CoMnO
6
shows better activity if compared with single perovskites due to high lattice oxygen content and good reducibility. Subsequently, perovskite catalysts are combined with plasma (NTP) to form in-plasma catalysis (IPC) and post-plasma catalysis (PPC) systems. The results indicate that IPC systems have better higher performance than that of NTP-alone and PPC. Especially, high C
7
H
8
conversion (100%) and mineralization efficiency (96.8%) can be achieved with the applied voltage of 18 kV and temperature of 120 °C when La
2
CoMnO
6
is integrated with NTP to form IPC system. Also, it owns the highest energy efficiency (0.14 g/kWh). It is concluded that IPC performance for C
7
H
8
removal is closely related with the properties of catalyst surface. In addition, the kinetics of IPC systems are investigated by a simplified model, and the result indicates that IPC with La
2
CoMnO
6
as catalyst has a higher overall energy constant. This study reveals that double-type La
2
CoMnO
6
is of higher activity than single perovskites for C
7
H
8
removal, and demonstrates that double-type La
2
CoMnO
6
is of high potential to form plasma catalysis system for VOCs removal.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-019-04714-0</identifier><identifier>PMID: 30895547</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Calcium Compounds - chemistry ; Catalysis ; Catalysts ; Catalytic oxidation ; Earth and Environmental Science ; Ecotoxicology ; Energy conversion efficiency ; Energy efficiency ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Lanthanum compounds ; Mineralization ; Oxidation ; Oxidation-Reduction ; Oxides - chemistry ; Oxygen content ; Perovskites ; Plasma ; Reaction kinetics ; Research Article ; Titanium - chemistry ; Toluene ; Toluene - chemistry ; Waste Water Technology ; Water Management ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2019-05, Vol.26 (13), p.12948-12962</ispartof><rights>Springer-Verlag GmbH Germany, part of Springer Nature 2019</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, (2019). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c412t-7b548e80dd6fd7f2a57912988a4ebf5808e28937c7d78b5b696f3900d625fd7d3</citedby><cites>FETCH-LOGICAL-c412t-7b548e80dd6fd7f2a57912988a4ebf5808e28937c7d78b5b696f3900d625fd7d3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-019-04714-0$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-019-04714-0$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/30895547$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Pan, Kuan Lun</creatorcontrib><creatorcontrib>Chang, Moo Been</creatorcontrib><title>Plasma catalytic oxidation of toluene over double perovskite-type oxide via packed-bed DBD</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Various perovskite-type catalysts including La
2
CoMnO
6
, LaCoO
3
, and LaMnO
3
are first evaluated for the activities toward C
7
H
8
removal. Experimental results indicate that double-type La
2
CoMnO
6
shows better activity if compared with single perovskites due to high lattice oxygen content and good reducibility. Subsequently, perovskite catalysts are combined with plasma (NTP) to form in-plasma catalysis (IPC) and post-plasma catalysis (PPC) systems. The results indicate that IPC systems have better higher performance than that of NTP-alone and PPC. Especially, high C
7
H
8
conversion (100%) and mineralization efficiency (96.8%) can be achieved with the applied voltage of 18 kV and temperature of 120 °C when La
2
CoMnO
6
is integrated with NTP to form IPC system. Also, it owns the highest energy efficiency (0.14 g/kWh). It is concluded that IPC performance for C
7
H
8
removal is closely related with the properties of catalyst surface. In addition, the kinetics of IPC systems are investigated by a simplified model, and the result indicates that IPC with La
2
CoMnO
6
as catalyst has a higher overall energy constant. This study reveals that double-type La
2
CoMnO
6
is of higher activity than single perovskites for C
7
H
8
removal, and demonstrates that double-type La
2
CoMnO
6
is of high potential to form plasma catalysis system for VOCs removal.</description><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Calcium Compounds - chemistry</subject><subject>Catalysis</subject><subject>Catalysts</subject><subject>Catalytic oxidation</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Energy conversion efficiency</subject><subject>Energy efficiency</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Lanthanum compounds</subject><subject>Mineralization</subject><subject>Oxidation</subject><subject>Oxidation-Reduction</subject><subject>Oxides - chemistry</subject><subject>Oxygen content</subject><subject>Perovskites</subject><subject>Plasma</subject><subject>Reaction kinetics</subject><subject>Research Article</subject><subject>Titanium - chemistry</subject><subject>Toluene</subject><subject>Toluene - chemistry</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp9kE1v1DAQhi1ERbeFP8ABWeLCxe3YsWP72O8iVYIDXLhYTjxBabNxaicr9t_X7RYqcejJI_l53xk9hHzkcMQB9HHmvFI1A24ZSM0lgzdkxesyaGntW7ICKyXjlZT75CDnWwABVuh3ZL8CY5WSekV-fR98Xnva-tkP27lvafzTBz_3caSxo3McFhyRxg0mGuLSDEgnTHGT7_oZ2byd8CmAdNN7Ovn2DgNrMNDz0_P3ZK_zQ8YPz-8h-Xl58ePsmt18u_p6dnLDWsnFzHSjpEEDIdRd0J3wSlsurDFeYtMpAwaFsZVuddCmUU1t666yAKEWqgRCdUi-7HqnFO8XzLNb97nFYfAjxiU7wa0StRDSFvTzf-htXNJYrnukpKyUEKJQYke1KeacsHNT6tc-bR0H92je7cy7Yt49mXdQQp-eq5dmjeFf5K_qAlQ7IJev8Teml92v1D4APveNgQ</recordid><startdate>20190501</startdate><enddate>20190501</enddate><creator>Pan, Kuan Lun</creator><creator>Chang, Moo Been</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QL</scope><scope>7SN</scope><scope>7T7</scope><scope>7TV</scope><scope>7U7</scope><scope>7WY</scope><scope>7WZ</scope><scope>7X7</scope><scope>7XB</scope><scope>87Z</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8FL</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BEZIV</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FRNLG</scope><scope>FYUFA</scope><scope>F~G</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K60</scope><scope>K6~</scope><scope>K9.</scope><scope>L.-</scope><scope>M0C</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7N</scope><scope>P64</scope><scope>PATMY</scope><scope>PQBIZ</scope><scope>PQBZA</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>7X8</scope></search><sort><creationdate>20190501</creationdate><title>Plasma catalytic oxidation of toluene over double perovskite-type oxide via packed-bed DBD</title><author>Pan, Kuan Lun ; Chang, Moo Been</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c412t-7b548e80dd6fd7f2a57912988a4ebf5808e28937c7d78b5b696f3900d625fd7d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Calcium Compounds - chemistry</topic><topic>Catalysis</topic><topic>Catalysts</topic><topic>Catalytic oxidation</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Energy conversion efficiency</topic><topic>Energy efficiency</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental science</topic><topic>Lanthanum compounds</topic><topic>Mineralization</topic><topic>Oxidation</topic><topic>Oxidation-Reduction</topic><topic>Oxides - chemistry</topic><topic>Oxygen content</topic><topic>Perovskites</topic><topic>Plasma</topic><topic>Reaction kinetics</topic><topic>Research Article</topic><topic>Titanium - chemistry</topic><topic>Toluene</topic><topic>Toluene - chemistry</topic><topic>Waste Water Technology</topic><topic>Water Management</topic><topic>Water Pollution Control</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Pan, Kuan Lun</creatorcontrib><creatorcontrib>Chang, Moo Been</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Bacteriology Abstracts (Microbiology B)</collection><collection>Ecology Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>ABI/INFORM Collection</collection><collection>ABI/INFORM Global (PDF only)</collection><collection>Health & Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>ABI/INFORM Global (Alumni Edition)</collection><collection>Medical Database (Alumni Edition)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest Pharma Collection</collection><collection>Public Health Database</collection><collection>Technology Research Database</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>ABI/INFORM Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>Agricultural & Environmental Science Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Business Premium Collection</collection><collection>Natural Science Collection</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>Engineering Research Database</collection><collection>Business Premium Collection (Alumni)</collection><collection>Health Research Premium Collection</collection><collection>ABI/INFORM Global (Corporate)</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Business Collection (Alumni Edition)</collection><collection>ProQuest Business Collection</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>ABI/INFORM Professional Advanced</collection><collection>ABI/INFORM Global</collection><collection>Health & Medical Collection (Alumni Edition)</collection><collection>Medical Database</collection><collection>Science Database</collection><collection>Algology Mycology and Protozoology Abstracts (Microbiology C)</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Environmental Science Database</collection><collection>ProQuest One Business</collection><collection>ProQuest One Business (Alumni)</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Environmental Science Collection</collection><collection>ProQuest Central Basic</collection><collection>MEDLINE - Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Pan, Kuan Lun</au><au>Chang, Moo Been</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Plasma catalytic oxidation of toluene over double perovskite-type oxide via packed-bed DBD</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2019-05-01</date><risdate>2019</risdate><volume>26</volume><issue>13</issue><spage>12948</spage><epage>12962</epage><pages>12948-12962</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Various perovskite-type catalysts including La
2
CoMnO
6
, LaCoO
3
, and LaMnO
3
are first evaluated for the activities toward C
7
H
8
removal. Experimental results indicate that double-type La
2
CoMnO
6
shows better activity if compared with single perovskites due to high lattice oxygen content and good reducibility. Subsequently, perovskite catalysts are combined with plasma (NTP) to form in-plasma catalysis (IPC) and post-plasma catalysis (PPC) systems. The results indicate that IPC systems have better higher performance than that of NTP-alone and PPC. Especially, high C
7
H
8
conversion (100%) and mineralization efficiency (96.8%) can be achieved with the applied voltage of 18 kV and temperature of 120 °C when La
2
CoMnO
6
is integrated with NTP to form IPC system. Also, it owns the highest energy efficiency (0.14 g/kWh). It is concluded that IPC performance for C
7
H
8
removal is closely related with the properties of catalyst surface. In addition, the kinetics of IPC systems are investigated by a simplified model, and the result indicates that IPC with La
2
CoMnO
6
as catalyst has a higher overall energy constant. This study reveals that double-type La
2
CoMnO
6
is of higher activity than single perovskites for C
7
H
8
removal, and demonstrates that double-type La
2
CoMnO
6
is of high potential to form plasma catalysis system for VOCs removal.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>30895547</pmid><doi>10.1007/s11356-019-04714-0</doi><tpages>15</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0944-1344 |
| ispartof | Environmental science and pollution research international, 2019-05, Vol.26 (13), p.12948-12962 |
| issn | 0944-1344 1614-7499 |
| language | eng |
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| source | MEDLINE; SpringerLink Journals - AutoHoldings |
| subjects | Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Calcium Compounds - chemistry Catalysis Catalysts Catalytic oxidation Earth and Environmental Science Ecotoxicology Energy conversion efficiency Energy efficiency Environment Environmental Chemistry Environmental Health Environmental science Lanthanum compounds Mineralization Oxidation Oxidation-Reduction Oxides - chemistry Oxygen content Perovskites Plasma Reaction kinetics Research Article Titanium - chemistry Toluene Toluene - chemistry Waste Water Technology Water Management Water Pollution Control |
| title | Plasma catalytic oxidation of toluene over double perovskite-type oxide via packed-bed DBD |
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