Inferential model estimates of ammonia dry deposition in the vicinity of a swine production facility
This project investigates NH 3 dry deposition around a commercial swine production facility in eastern North Carolina. Passive diffusion-tube samplers were used to measure weekly integrated NH 3 concentrations at 22 locations along horizontal gradients from the barn/lagoon emissions complex (source)...
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Veröffentlicht in: | Atmospheric environment (1994) 2008-05, Vol.42 (14), p.3407-3418 |
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Format: | Artikel |
Sprache: | eng |
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Zusammenfassung: | This project investigates NH
3 dry deposition around a commercial swine production facility in eastern North Carolina. Passive diffusion-tube samplers were used to measure weekly integrated NH
3 concentrations at 22 locations along horizontal gradients from the barn/lagoon emissions complex (source) out to a distance of 700
m. A two-layer canopy compensation point model was used to predict bi-directional NH
3 exchange within a 500
m circular buffer surrounding the source. The model takes into account differences in soil and vegetation emission potential, as well as canopy physical characteristics, among three primary surfaces surrounding the site: forest, crops spray fertilized with swine waste, and other fertilized crops. Between June 2003 and July 2005, mean observed NH
3 concentrations ranged from 169.0
μg NH
3
m
−3 at a distance of 10
m from the source to 7.1 and 13.0
μg NH
3
m
−3 at 612 and 698
m in the predominant upwind and downwind directions, respectively. Median predicted dry deposition rates ranged from 145
kg NH
3–N
ha
−1
yr
−1 at 10
m from the source to 16
kg NH
3–N
ha
−1
yr
−1 at 500
m, which is ≈3.5× wet deposition of NH
4
+–N. Assuming a steady-state emission factor of 7.0
kg NH
3
animal
−1
yr
−1 and a median population of 4900 animals, NH
3 dry deposition over the nearest 500
m from the barn/lagoon complex accounted for 10.4% (3567
kg NH
3) of annual emissions (34,300
kg
NH
3). A model sensitivity analysis shows that predicted deposition rates are more sensitive to assumptions regarding cuticular uptake relative to soil and vegetation emission potentials. |
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ISSN: | 1352-2310 1873-2844 |
DOI: | 10.1016/j.atmosenv.2007.06.004 |